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We survey our research on modeling the mechanisms of control of uniformity in growth of nanosize and colloid particles. The former are produced as nanocrystals, by burst-nucleation from solution. The latter, colloid-size particles, are…

Soft Condensed Matter · Physics 2010-10-12 Vladimir Privman

We review theoretical explanation of mechanisms of control of uniformity in growth of nanosize particles and colloids. The nanoparticles are synthesized as nanocrystals, by burst nucleation from solution. The colloids are self-assembled by…

Statistical Mechanics · Physics 2010-09-22 Vladimir Privman

We report numerical investigations of a three-dimensional model of diffusive growth of fine particles, the internal structure of which corresponds to different crystal lattices. A growing cluster (particle) is immersed in, and exchanges…

Statistical Mechanics · Physics 2010-10-12 Vyacheslav Gorshkov , Alexandr Zavalov , Vladimir Privman

We study the nucleation of crystalline cluster phases in the generalized exponential model with exponent n=4. Due to the finite value of this pair potential for zero separation, at high densities the system forms cluster crystals with…

Soft Condensed Matter · Physics 2016-09-01 Christian Leitold , Christoph Dellago

Crystal nucleation and growth processes induced by an externally applied shear strain in a model metallic glass are studied by means of nonequilibrium molecular dynamics simulations, in a range of temperatures. We observe that the…

Materials Science · Physics 2010-09-30 Anatolii Mokshin , J. -L. Barrat

A mathematical model to describe the growth of an arbitrarily large number of nanocrystals from solution is presented. First, the model for a single particle is developed. By non-dimensionalising the system we are able to determine the…

Mesoscale and Nanoscale Physics · Physics 2020-11-17 C. Fanelli , V. Cregan , F. Font , T. G. Myers

State-of-the-art models for aerosol particle nucleation and growth from a cooling vapor primarily use a nodal method to numerically solve particle growth kinetics. In this method, particles that are smaller than the critical size are…

Computational Physics · Physics 2024-08-30 A. Khrabry , I. D. Kaganovich , S. Raman , E. Turkoz , D. Graves

Under continuous laser irradiation, noble metal nanoparticles immersed in water can quickly heat up, leading to the nucleation of so-called plasmonic bubbles. In this work, we want to further understand the bubble nucleation and growth…

The nucleation and growth of clusters in a progressively cooled vapor is studied. The chemical-potential of the vapor increases, resulting in a rapidly increasing nucleation rate. The growth of the newly created clusters depletes monomers,…

Materials Science · Physics 2008-10-21 Yossi Farjoun

This paper presents a comprehensive analysis of simple models useful to analyze the growth of nanostructures obtained by cluster deposition. After detailing the potential interest of nanostructures, I extensively study the first stages of…

Materials Science · Physics 2015-06-25 Pablo Jensen

The time-dependent kinetics of formation and evolution of nano-size atomic clusters is investigated and illustrated with the nucleation dynamics of ion-seed Ar$_n$H$^+$ particles. The rates of growth and degradation of Ar-atomic shells…

Atomic and Molecular Clusters · Physics 2022-02-23 M. G. Rozman , M. Bredice , J. Smucker , H. R. Sadeghpour , D. Vrinceanu , R. Cote , V. Kharchenko

When dissipative particles are left alone, their fluctuation energy decays due to collisional interactions, clusters build up and grow with time until the system size is reached. When the effective dissipation is strong enough, this may…

Statistical Mechanics · Physics 2009-10-31 S. Luding , H. J. Herrmann

We study the coalescence of nanoscale metal clusters in an inert-gas atmosphere using constant-energy molecular dynamics. The coalescence proceeds via atomic diffusion with the release of surface energy raising the temperature. If the…

Condensed Matter · Physics 2007-05-23 Shaun C. Hendy , Simon A. Brown , Michael Hyslop

We study the conditions under which and how an imposed cluster of fixed colloidal particles at prescribed positions triggers crystal nucleation from a metastable colloidal fluid. Dynamical density functional theory of freezing and Brownian…

Soft Condensed Matter · Physics 2009-11-13 Sven van Teeffelen , Christos N. Likos , Hartmut Löwen

The appearance of nuclear clusters in stellar matter at densities below nuclear saturation is an important feature in the modeling of the equation of state for astrophysical applications. There are different theoretical concepts to describe…

Nuclear Theory · Physics 2016-12-22 Helena Pais , Stefan Typel

The diffusion and coalescence of individual atoms on a nanostructured surface are treated in a purely statistical way. From this, analytical formulas are derived which, from a known initial state, give the final cluster size distribution on…

Statistical Mechanics · Physics 2021-03-16 Georges Sitja

We have performed large-scale Lennard-Jones molecular dynamics simulations of homogeneous vapor-to-liquid nucleation, with $10^9$ atoms. This large number allows us to resolve extremely low nucleation rates, and also provides excellent…

Chemical Physics · Physics 2014-04-07 Raymond Angélil , Jürg Diemand , Kyoko K. Tanaka , Hidekazu Tanaka

The premelting plays an important role in ice growth, but there is a significant gap in our knowledge between the atomistic premelting surface structure and the macroscopic growth mechanism. In this work, using large-scale molecular…

Chemical Physics · Physics 2022-11-04 Shifan Cui , Haoxiang Chen , Zhengpu Zhao

We propose a new method of estimating the mean diameter and dispersion of clusters formed in a cooling gas, right after the nucleation stage. Using a moment model developed by Friedlander [S.K. Friedlander, Ann. N.Y. Acad. Sci. 354 (1983)],…

Soft Condensed Matter · Physics 2020-08-19 Mikael Tacu , Alexander Khrabry , Igor Kaganovich

During the processes of nucleation and growth of a precipitate cluster from a supersaturated solution, the diffusion flux between the cluster and the solution changes the solute concentration near the cluster-solution interface from its…

Chemical Physics · Physics 2016-06-08 Alexander Borisenko
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