Related papers: Interplay of polarization geometry and rotational …
Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular…
The polarization state of light plays a central role in strong-field light--matter interactions and is widely used to probe electronic structure in solids via high-order harmonic generation (HHG). In particular, helicity-resolved HHG has…
We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…
Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…
We study intraband high-order harmonic generation arising from a band-gap material driven by a linearly polarized laser field. We factorize the intraband high-order harmonic-generation signal into intracycle and intercycle terms. The…
The Letter is devoted to new frequencies generation and its role in the synchronization of two spatially separated polariton condensates affected by the coherent pump with the frequency detuned from the frequencies of the condensates. We…
We demonstrate theoretically and experimentally coherence-induced polarization changes in generic and higher-order vector vortex beams with polarization singularity. The prominent depolarization on decreasing transverse correlation-width in…
The influence of the orbital symmetry on the ellipticity of the high-order harmonics is investigated. It is found that the ellipticity maps have distinct shapes for the molecular orbital with different symmetry. Our analysis shows that the…
We present a new theory that the molecular high order harmonic generation in an intense laser field is determined by molecular internal symmetry and momentum distribution of the tunneling-ionized electron. The molecular internal symmetry…
The objective of this article is to investigate the profound nonlinear optical response exhibited by inversion symmetric fullerene molecules under the influence of different types of disorders described by the Anderson model. Our aim is to…
High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…
We explore pump-probe high harmonic generation (HHG) from monolayer hexagonal-Boron-Nitride, where a terahertz pump excites coherent optical phonons that are subsequently probed by an intense infrared pulse that drives HHG. We find, through…
High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…
Topological materials are of interest to both fundamental science and advanced technologies, because topological states are robust with respect to perturbations and dissipation. Experimental detection of topological invariants is thus in…
We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…
The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…
We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…
We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…
Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…
We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…