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We have computed the surface energies, work functions, and interlayer surface relaxations of clean (111), (110), and (100) surfaces of Al, Cu, Ru, Rh, Pd, Ag, Pt, and Au. Many of these metallic surfaces have technological or catalytic…

Materials Science · Physics 2022-06-01 Abhirup Patra , Jefferson E. Bates , Jianwei Sun , John P. Perdew

Generalized Advantage Estimation (GAE) has been used to mitigate the computational complexity of reinforcement learning (RL) by employing an exponentially weighted estimation of the advantage function to reduce the variance in policy…

Machine Learning · Computer Science 2025-07-24 Shahil Shaik , Jonathon M. Smereka , Yue Wang

We derive and motivate a Laplacian-level, orbital-free meta-generalized-gradient approximation (LL-MGGA) for the exchange-correlation energy, targeting accurate ground-state properties of $sp$ and $sd$ metallic condensed matter, in which…

Materials Science · Physics 2022-08-02 Aaron D. Kaplan , John P. Perdew

This paper introduces a novel family of generalized exponentiated gradient (EG) updates derived from an Alpha-Beta divergence regularization function. Collectively referred to as EGAB, the proposed updates belong to the category of…

Machine Learning · Computer Science 2024-12-30 Andrzej Cichocki , Sergio Cruces , Auxiliadora Sarmiento , Toshihisa Tanaka

A tutorial introduction to projective geometric algebra (PGA), a modern, coordinate-free framework for doing euclidean geometry. PGA features: uniform representation of points, lines, and planes; robust, parallel-safe join and meet…

General Mathematics · Mathematics 2020-08-19 Charles G. Gunn

The bulk properties (lattice constants, bulk moduli, and cohesive energies) of alkali, alkaline-earth, and transition metals are studied within the framework of the recently developed meta-GGA (meta-Generalized Gradient Approximation)…

Materials Science · Physics 2018-11-14 Subrata Jana , Kedar Sharma , Prasanjit Samal

Meta-generalized gradient approximations (meta-GGAs) on the third rung of the functional hierarchy are gaining increasing relevance for the electronic structure. Meta-GGAs are constructed from numerous ingredients including the orbital…

Materials Science · Physics 2025-06-05 Ashesh Giri , Chandra Shahi , Adrienn Ruzsinszky

It is known that the adiabatic approximation in time-dependent density functional theory usually provides a good description of low-lying excitations of molecules. In the present work, the capability of the adiabatic nonempirical…

Materials Science · Physics 2009-11-13 Jianmin Tao , Sergei Tretiak , Jian-Xin Zhu

The proximal gradient method is a generic technique introduced to tackle the non-smoothness in optimization problems, wherein the objective function is expressed as the sum of a differentiable convex part and a non-differentiable…

Numerical Analysis · Mathematics 2024-01-19 Abdeslem Hafid Bentbib , Khalide Jbilou , Ridwane Tahiri

Learning PDE dynamics for fluids increasingly relies on neural operators and Transformer-based models, yet these approaches often lack interpretability and struggle with localized, high-frequency structures while incurring quadratic cost in…

Machine Learning · Computer Science 2026-02-26 Zhihao Li , Yu Feng , Zhilu Lai , Wei Wang

Proximal gradient algorithms (PGA), while foundational for inverse problems like image reconstruction, often yield unstable convergence and suboptimal solutions by violating the critical non-negativity constraint. We identify the gradient…

Machine Learning · Computer Science 2025-10-28 Hanzhang Wang , Zonglin Liu , Jingyi Xu , Chenyang Wang , Zhiwei Zhong , Qiangqiang Shen

We present a uniform analysis of biased stochastic gradient methods for minimizing convex, strongly convex, and non-convex composite objectives, and identify settings where bias is useful in stochastic gradient estimation. The framework we…

Optimization and Control · Mathematics 2020-02-28 Derek Driggs , Jingwei Liang , Carola-Bibiane Schönlieb

A procedure for removing explicit orbital dependence from meta-generalized-gradient approximation (mGGA) exchange-correlation functionals by converting them into Laplacian-dependent functionals recently was developed by us and shown to be…

Materials Science · Physics 2018-10-03 Daniel Mejia-Rodriguez , S. B. Trickey

This paper presents an Accelerated Preconditioned Proximal Gradient Algorithm (APPGA) for effectively solving a class of Positron Emission Tomography (PET) image reconstruction models with differentiable regularizers. We establish the…

Optimization and Control · Mathematics 2024-09-23 Yizun Lin , Yongxin He , C. Ross Schmidtlein , Deren Han

Generalized Hydrodynamics (GHD) has recently been devised as a method to solve the dynamics of integrable quantum many-body systems beyond the mean-field approximation. In its original form, a major limitation is the inability to predict…

The generalized eigenvalue problem (GEP) serves as a cornerstone in a wide range of applications in numerical linear algebra and scientific computing. However, traditional approaches that aim to maximize the classical Rayleigh quotient…

Optimization and Control · Mathematics 2025-07-04 Xiaozhi Liu , Yong Xia

We consider adaptive finite element methods (AFEMs) with inexact algebraic solvers for second-order symmetric linear elliptic diffusion problems. Optimal complexity of AFEM, i.e., optimal convergence rates with respect to the overall…

Numerical Analysis · Mathematics 2026-04-10 Paula Hilbert , Ani Miraçi , Dirk Praetorius

We propose a tensor-based criterion for benign landscape in phase retrieval and establish boundedness of gradient trajectories. This implies that gradient descent will converge to a global minimum for almost every initial point.

Optimization and Control · Mathematics 2024-10-18 Théodore Fougereux , Cédric Josz , Xiaopeng Li

Using a reverse-engineering method we construct a meta-generalized gradient approximation (meta-GGA) angle-averaged exchange-correlation hole model which has a general applicability. It satisfies known exact hole constraints and can exactly…

Chemical Physics · Physics 2013-09-17 L. A. Constantin , E. Fabiano , F. Della Sala

The parquet formalism and Hedin's $GW\gamma$ approach are unified into a single theory of vertex corrections, corresponding to an exact reformulation of the parquet equations in terms of boson exchange. The method has no drawbacks compared…

Strongly Correlated Electrons · Physics 2021-02-25 Friedrich Krien , Anna Kauch , Karsten Held