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Local dielectric spectroscopy is performed to study how relaxation dynamics of a poly-vinyl-acetate ultra-thin film is influenced by inorganic nano-inclusions of a layered silicate (montmorillonite). Dielectric loss spectra are measured by…

Using non-contact scanning probe microscopy (SPM) techniques, dielectric properties were studied on 50 nanometer length scales in poly-vinyl-acetate (PVAc) films in the vicinity of the glass transition. Low frequency (1/f) noise observed in…

Disordered Systems and Neural Networks · Physics 2009-10-31 E. Vidal Russell , N. E. Israeloff , L. E. Walther , H. Alvarez Gomariz

Dielectric relaxation and thermal expansion spectroscopy were made for thin polystyrene films in order to measure the temperature $T_{\alpha}$ corresponding to the peak in the loss component of susceptibility due to the $\alpha$-process and…

Soft Condensed Matter · Physics 2007-05-23 Koji Fukao , Yoshihisa Miyamoto

Dynamics of thin films of poly(vinyl acetate) (PVAc) and poly(methyl methacrylate) (PMMA) have been investigated by dielectric relaxation spectroscopy in the frequency range from 0.1Hz to 1MHz at temperatures from 263K to 423K. The…

Soft Condensed Matter · Physics 2009-11-07 Koji Fukao , Shinobu Uno , Yoshihisa Miyamoto , Akitaka Hoshino , Hideki Miyaji

The glass transition temperature and relaxation dynamics of the segmental motions of thin films of polystyrene labeled with a dye, 4-[N-ethyl-N-(hydroxyethyl)]amino-4-nitraozobenzene (Disperse Red 1, DR1) are investigated using dielectric…

Soft Condensed Matter · Physics 2009-11-13 Rodney D. Priestley , Linda J. Broadbelt , John M. Torkelson , Koji Fukao

The glass transition temperature $T_{\rm g}$ and the temperature $T_{\alpha}$ corresponding to the peak in the dielectric loss due to the $\alpha$-process have been simultaneously determined as functions of film thickness d through…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

Dielectric spectroscopy measurements over a broad range of temperature and pressure were carried out on poly(oxybutylene) (POB), a type-A polymer (dielectrically-active normal mode). There are three dynamic processes appearing at lower…

Soft Condensed Matter · Physics 2009-11-10 R. Casalini , C. M. Roland

We present the high pressure dielectric spectroscopy (up to 4.2 GPa) and ultrasonic study (up to 1.7 GPa) of liquid and glassy propylene carbonate (PC). Both of the methods provide complementary pictures of the glass transition in PC under…

Soft Condensed Matter · Physics 2013-05-17 M. V. Kondrin , E. L. Gromnitskaya , A. A. Pronin , A. G. Lyapin , V. V. Brazhkin , A. A. Volkov

The $\alpha$-process (segmental motion) of thin polystyrene films supported on glass substrate has been investigated in a wider frequency range from 10$^{-3}$ Hz to 10$^4$ Hz using dielectric relaxation spectroscopy and thermal expansion…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

We investigate the relaxation behavior of thin films of a polyamide random copolymer, PA66/6I, with various film thicknesses using dielectric relaxation spectroscopy. Two dielectric signals are observed at high temperatures, the…

Soft Condensed Matter · Physics 2015-06-11 Natsumi Taniguchi , Koji Fukao , Paul Sotta , Didier R. Long

We measure the isothermal rejuvenation of stable glass films of poly(styrene) and poly(methylmethacrylate). We demonstrate that the propagation of the front responsible for the transformation to a supercooled-liquid state can serve as a…

Soft Condensed Matter · Physics 2023-12-12 Saba Karimi , Junjie Yin , Thomas Salez , James A Forrest

Poly(vinyl alcohol)/Poly(vinylidene fluoride) blends at mass ratio 3:1 with Nano - Graphene Platelet fillers constitute mechanically and thermally stable systems, which are used for developing piezoelectric devices. Blends host a fraction…

Chemical Physics · Physics 2025-05-07 Eirini Kolonelou , Anthony N. Papathanassiou

The polymer relaxation dynamic of a sample, stretched up to the stress hardening regime, is measured, at room temperature, as a function of the strain $\lambda$ for a wide range of the strain rate $\dot\gamma$, by an original dielectric…

Soft Condensed Matter · Physics 2020-03-11 R. Sahli , J. Hem , C. Crauste-Thibierge , F. Clément , D Long , S. Ciliberto

An analysis of the glass transition of four materials with similar chemical structures is performed: PET, PEN and two PET/PEN blends (90/10 and 70/30 w/w). During the melt processing of the blends transesterification reactions yield block…

Materials Science · Physics 2015-06-05 J. Sellares , J. A. Diego , J. C. Canadas , M. Mudarra , J. Belana , P. Colomer , F. Roman , Y. Calventus

Dielectric spectroscopy is one of the most commonly used techniques for the investigation of the dynamic response of glass-forming materials. The tremendous slow-down of the particle motions when approaching the glass transition and…

Disordered Systems and Neural Networks · Physics 2007-05-23 U. Schneider , P. Lunkenheimer , A. Pimenov , R. Brand , A. Loidl

The glass transition temperature $T_g$ and the temperature $T_{\alpha}$ corresponding to the peak in the dielectric loss due to the $\alpha$-process have been simultaneously determined as functions of film thickness $d$ through dielectric…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

Dielectric relaxation spectroscopy 10^-1 Hz to 10^6 Hz) is employed to study the molecular dynamics of poly(dimethylsiloxane) (PDMS, Mw=1.7 10^5 g/mol and Mw=9.6 10^4 g/mol as grafted films with thicknesses d below and above the radius of…

Soft Condensed Matter · Physics 2009-11-07 L. Hartmann , P. Pouret , L. Leger , F. Kremer

Complex permittivity studies on glassy poly(vinyl alcohol)/poly(vinyl pyrrolidone) (1/1) at proper pressure-temperature condition, provide the activation volume and energy values for both dc conductivity and \b{eta}-relaxation. The…

Materials Science · Physics 2018-11-01 Eirini Kolonelou , Anthony N. Papathanassiou , Elias Sakellis

We report a thorough dielectric characterization of the alpha relaxation of glass forming glycerol with varying additions of LiCl. Nine salt concentrations from 0.1 - 20 mol% are investigated in a frequency range of 20 Hz - 3 GHz and…

Soft Condensed Matter · Physics 2008-10-29 M. Köhler , P. Lunkenheimer , A. Loidl

Shear-mechanical and dielectric measurements on the two monohydroxy (mono-alcohol) molecular glass formers 2-ethyl-1-hexanol and 2-butanol close to the glass transition temperature are presented. The shear-mechanical data are obtained using…

Soft Condensed Matter · Physics 2008-11-14 Bo Jakobsen , Claudio Maggi , Tage Christensen , Jeppe C. Dyre
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