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We introduce two simple models with nearest neighbor interactions on 3D hexagonal lattices. Each model allows one to calculate the residual entropy of ice I (ordinary ice) by means of multicanonical simulations. This gives the correction to…

Statistical Mechanics · Physics 2013-05-29 Bernd A. Berg , Chizuru Muguruma , Yuko Okamoto

The configurational entropy of ice is calculated by thermodynamic integration from high to low temperatures. We use Monte Carlo simulations with a simple energy model which reproduces the Bernal-Fowler ice rules. This procedure is found to…

Chemical Physics · Physics 2015-06-16 Carlos P. Herrero , Rafael Ramirez

The configurational entropy of several H-disordered ice polymorphs is calculated by means of a thermodynamic integration along a path between a totally H-disordered state and one fulfilling the Bernal-Fowler ice rules. A Monte Carlo…

Chemical Physics · Physics 2014-06-24 Carlos P. Herrero , Rafael Ramirez

We estimated the residual entropy of ice Ih by the recently developed simulation protocol, namely, the combination of Replica-Exchange Wang-Landau algorithm and Multicanonical Replica-Exchange Method. We employed a model with the nearest…

Statistical Mechanics · Physics 2021-02-24 Takuya Hayashi , Chizuru Muguruma , Yuko Okamoto

Computer simulations have been employed in recent years to evaluate the configurational entropy changes in model glass-forming liquids. We consider two methods, both of which involve the calculation of the `intra-basin' entropy as a means…

Statistical Mechanics · Physics 2009-10-31 Srikanth Sastry

Characterizing the entropy of a system is a crucial, and often computationally costly, step in understanding its thermodynamics. It plays a key role in the study of phase transitions, pattern formation, protein folding and more. Current…

Statistical Mechanics · Physics 2020-12-02 Amit Nir , Eran Sela , Roy Beck , Yohai Bar-Sinai

The problems of conditional entropy's definition and the formula to compute conditional entropy are analyzed from various perspectives, and the corrected computing formula is presented. Examples are given to prove the conclusion that…

Information Theory · Computer Science 2007-08-24 Wang Yong

Stable numerical simulations for a hyperbolic system of conservation laws of relaxation type but not in divergence form are obtained by incorporating the physical entropy into the simulations. The entropy balance is utilized as an…

Numerical Analysis · Mathematics 2019-01-10 Carl Philipp Zinner , Hans Christian Öttinger

We present a recursive procedure to calculate the parameters of the recently introduced multicanonical ensemble and explore the approach for spin glasses. Temperature dependence of the energy, the entropy and other physical quantities are…

High Energy Physics - Lattice · Physics 2009-01-23 Bernd A. Berg , Tarik Celik

We investigate how the temperature calculated from the microcanonical entropy compares with the canonical temperature for finite isolated quantum systems. We concentrate on systems with sizes that make them accessible to numerical exact…

Statistical Mechanics · Physics 2023-04-05 Phillip C. Burke , Masudul Haque

Firstly, we calculate quantitatively decrease of entropy by the known formulas in the ordering phenomena and nucleation of thermodynamics of microstructure. They show again that a necessary condition of decrease of entropy in isolated…

General Physics · Physics 2009-05-04 Yi-Fang Chang

Polydisperse systems are commonly encountered when dealing with soft matter in general or any non simple fluid. Yet their treatment within the framework of statistical thermodynamics is a delicate task as the latter has been essentially…

Statistical Mechanics · Physics 2015-06-22 Fabien Paillusson , Ignacio Pagonabarraga

Comparison-based algorithms are algorithms for which the execution of each operation is solely based on the outcome of a series of comparisons between elements. Comparison-based computations can be naturally represented via the following…

Data Structures and Algorithms · Computer Science 2020-11-17 Michel Schellekens

We propose a method for computing the Kolmogorov-Sinai (KS) entropy of chaotic systems. In this method, the KS entropy is expressed as a statistical average over the canonical ensemble for a Hamiltonian with many ground states. This…

Statistical Mechanics · Physics 2007-05-23 Shin-ichi Sasa , Kumiko Hayashi

From thermodynamic origins, the concept of entropy has expanded to a range of statistical measures of uncertainty, which may still be thermodynamically significant. However, laboratory measurements of entropy continue to rely on direct…

Statistical Mechanics · Physics 2012-04-24 Paul E. Lammert , Xianglin Ki , Jie Li , Cristiano Nisoli , David M. Garand , Vincent H. Crespi , Peter Schiffer

Several approximations are made to study the microcanonical formalism that are valid in the thermodynamics limit. Usually it is assumed that: 1)Stirling approximation can be used to evaluate the number of microstates; 2) the surface entropy…

General Physics · Physics 2015-10-07 E. N. Miranda , Dalia S. Bertoldi

The entropy is a measure of uncertainty that plays a central role in information theory. When the distribution of the data is unknown, an estimate of the entropy needs be obtained from the data sample itself. We propose a semi-parametric…

Methodology · Statistics 2022-01-06 Stéphane Robin , Luca Scrucca

In this paper we prove estimates on the behaviour of the Kolmogorov-Sinai entropy relative to a partition for randomly perturbed dynamical systems. Our estimates use the entropy for the unperturbed system and are obtained using the notion…

Dynamical Systems · Mathematics 2007-05-23 Claudio Bonanno

The paper analyzes the entropy of a system composed by non-interacting and indistinguishable particles whose quantum state numbers are modelled as independent and identically distributed classical random variables. The crucial observation…

Statistical Mechanics · Physics 2023-05-18 Arnaldo Spalvieri

Correlations reduce the configurational entropies of liquids below their ideal gas limits. By means of first principles molecular dynamics simulations, we obtain accurate pair correlation functions of liquid metals, then subtract the mutual…

Statistical Mechanics · Physics 2018-02-22 M. C. Gao , M. Widom
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