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We derive four sum-rule expressions for spectra measured in electron energy-loss near edge structure experiments. These sum-rules permit the determination spin and orbital magnetic moments, spin-orbit interaction and number of states,…

Materials Science · Physics 2009-11-13 Ján Rusz , Olle Eriksson , Pavel Novák , Peter M. Oppeneer

In this work we derive sum rules for orbital angular momentum(OAM) resolved electron magnetic chiral dichroism (EMCD) which enable the evaluation of the strength of spin and orbital components of the atomic magnetic moments in a crystalline…

It is proven that the sum rules for X-ray magnetic dichroism (XMCD) spectra that are used to separate spin and orbital contributions to the magnetic moment are formally correct for an arbitrary strength of electron-electron interactions.…

Strongly Correlated Electrons · Physics 2007-05-23 V. Yu. Irkhin , M. I. Katsnelson

Understanding the ramifications of reduced crystalline symmetry on magnetic behavior is a critical step in improving our understanding of nanoscale and interfacial magnetism. However, investigations of such effects are often controversial…

Electron magnetic chiral dichroism (EMCD) is an emerging tool for quantitative measurements of magnetic properties using the transmission electron microscope (TEM), with the possibility of nanometer resolution. The geometrical conditions,…

One of the most challenging issues in the characterization of magnetic materials is to obtain quantitative analysis on the nanometer scale. Here we describe how electron magnetic circular dichroism (EMCD) measurements using the transmission…

Recently it was demonstrated (Schattschneider et al., Nature 441 (2006), 486), that an analogue of the X-ray magnetic circular dichroism (XMCD) experiment can be performed with the transmission electron microscope (TEM). The new phenomenon…

Materials Science · Physics 2009-09-29 Jan Rusz , Stefano Rubino , Peter Schattschneider

We propose a highly efficient atomically-resolved mode of electron magnetic chiral dichroism. This method exploits the recently introduced orbital angular momentum spectrometer to analyze the inelastically scattered electrons allowing for…

We demonstrate electron magnetic linear dichroism as a quantitative probe of vectorial magnetic order parameters with nanometer resolution in transmission electron microscopy. Explicit inclusion of vectorial core-level exchange splitting…

Mesoscale and Nanoscale Physics · Physics 2026-05-28 Jan Hajduček , Jáchym Štindl , Ján Rusz , Vojtěch Uhlíř

A systematic ab initio study is performed for the spin and orbital moments and for the validity of the sum rules for x-ray magnetic circular dichroism for Fe systems with various dimensionality (bulk, Pt-supported monolayers and monatomic…

Materials Science · Physics 2009-11-10 Claude Ederer , Matej Komelj , Manfred Faehnle

We consider the magnetic circular dichroism spectrum of a crystal with broken time-reversal symmetry in the electric-dipole approximation. Using the Kubo-Greenwood formula for the absorptive part of the antisymmetric optical conductivity,…

Materials Science · Physics 2009-11-13 Ivo Souza , David Vanderbilt

Energy-loss magnetic chiral dichroism (EMCD) allows for the quantification of magnetic properties of materials at the nanometer scale. It is shown that with the support of simulations that help to identify the optimal conditions for a…

We derive a sum rule to demonstrate that the static magnetoelectric (ME) effect is governed by optical transitions that are simultaneously excited via the electric and magnetic components of light. By a systematic analysis of magnetic point…

Materials Science · Physics 2014-01-15 D. Szaller , S. Bordacs , V. Kocsis , U. Nagel , T. Room , I. Kezsmarki

In the highly non-equilibrium conditions of laser induced spin dynamics magnetic moments can only be obtained from the spectral information, most commonly from the spectroscopy of semi-core states using the so-called x-ray magnetic circular…

Materials Science · Physics 2021-04-05 S. Shallcross , J. K. Dewhurst , P. Elliott , S. Eisebitt , C. von Korff Schmising , S. Sharma

A detailed theoretical study on the electronic structure and magnetic properties of half-metallic ferromagnet CrO$_2$ was carried out by means of relativistic full-potential linear muffin-tin orbital method within the generalized gradient…

Materials Science · Physics 2009-11-11 V. Kanchana , G. Vaitheeswaran , M. Alouani

The electric-field control of $d$-electron magnetism in multiferroic transition metal oxides is attracting widespread interest for the underlying fundamental physics and for next generation spintronic devices. Here, we report an extensive…

Materials Science · Physics 2021-05-26 D. Preziosi , S. Homkar , C. Lefevre , M. Salluzzo , N. Viart

A light beam can carry both spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is commonly evidenced by circular dichroism (CD) experiments {\em i. e.} differential absorption of left and right-handed circularly polarized…

Electron magnetic circular dichroism (EMCD) in transmission electron microscopy (TEM) enables element-specific measurement of spin and orbital magnetic moments, analogous to X-ray magnetic circular dichroism (XMCD). While the EMCD technique…

We have measured the circular magnetic dichroism in the x-ray absorption at the K-edge of oxygen in microcrystals of different spinel oxides. The microcrystals are islands of micrometric size and nanometric thickness, grown on Ru(0001)…

The emergence of optical circular dichroism in chiral nanoscale and molecular systems provides not only a way for analyzing the sample chirality itself but also additional degrees of freedom in manipulating light. Such manipulation can be…

Mesoscale and Nanoscale Physics · Physics 2026-02-18 Marek Zálešák , Martin Ošmera , Martin Hrtoň , Andrea Konečná
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