Related papers: Selection of dominant multi-exciton transitions in…
We study the nonlinear optical response of argon to a four-wave-mixing pulse sequence consisting of an extreme ultraviolet pulse, an overlapping collinear IR and an non-collinear delayed IR pulses. Absorption of an extreme ultraviolet and…
We investigate globally coupled stochastic three-state oscillators, which we consider as general models of stochastic excitable systems. We compare two situations:in the first case the transitions between the three states of each unit…
In this article, we use a many-body approach to study the absorption spectra of electron-doped two-dimensional semiconductors. Optical absorption is modeled by a many-body scattering Hamiltonian which describes an exciton immersed in a…
The flux-based statistical theory of the non-hierarchical three-body system predicts that the chaotic outcome distribution reduces to the chaotic emissivity function times a known function, the asymptotic flux. Here, we measure the chaotic…
Third order parametric down-conversion describes a class of nonlinear processes in which a pump photon can be down-converted into triplets of photons. It has been identified as a source of non-classical light, with capabilities beyond those…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
Nonlinear responses of superconductors to intense terahertz radiation has been an active research frontier. Using terahertz pump-terahertz probe spectroscopy, we investigate the c-axis nonlinear optical response of a high-temperature…
Optical spectra of two-dimensional transition-metal dichalcogenides (TMDC) are influenced by complex multi-particle excitonic states. Their theoretical analysis requires solving the many-body problem, which in most cases, is prohibitively…
We characterize the optical response of a three-level atom subjected to an incoherent pump and continuously illuminated with a weak, quasi-resonant probe field. To this end, we apply a wavefunction approach based on QED Hamiltonian…
Absorption is usually expected to be detrimental to quantum coherence effects. However, the situation for complex absorption spectra has been little studied yet. We consider the resonance fluorescence of excitons in a semiconductor quantum…
In their Letter [Phys. Rev. Lett. 105, 137402 (2010)], Eisfeld et al. predicted the exchange broadening and blue-shift of the absorption band as well as a nonuniversal disorder scaling of the localization length of excitons in J-aggregates…
We report a numerical calculation of the total number of disordered jammed configurations $\Omega$ of $N$ repulsive, three-dimensional spheres in a fixed volume $V$. To make these calculations tractable, we increase the computational…
We apply low temperature confocal optical microscopy to spatially resolve, and spectroscopically study a single self assembled quantum dot. By comparing the emission spectra obtained at various excitation levels to a theoretical many body…
Recent experiments in the cuprates have seen evidence of a transient superconducting state upon optical excitation polarized along the c-axis [R. Mankowsky et al., Nature 516, 71 (2014)]. Motivated by these experiments we propose an…
The effect of an ac modulation on a 2-level or 3-level system is studied theoretically. The absorption spectrum is calculated by solving the optical Bloch equations and is interpreted by reference to the Floquet quasienergy spectrum. The…
The optical absorption spectrum of the three most stable isomers of the Ag11 system was calculated using the time-dependent density functional theory, with the generalized gradient approximation for the exchange and correlation potential,…
The properties of the absorbing states of non-equilibrium models belonging to the conserved directed percolation universality class are studied. We find that at the critical point the absorbing states are hyperuniform, exhibiting…
The optical response of a heavily doped quantum well, with two occupied subbands, has been investigated as a function of the electronic density. It is shown that the two optically active transitions are mutually coupled by dipole-dipole…
The interaction of laser radiation with single J aggregates of cyanine dyes is theoretically analyzed and numerically simulated. The quantum mechanical calculations of the equilibrium geometry and the energies and intensities of the lowest…
A general multiband formulation of linear and non-linear optical response functions for realistic models of correlated crystals is presented. Dipole forbidden d-d optical transitions originate from the vertex functions, which we consider…