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We present current-voltage (I-V) curves computed using all-electron basis sets on the conducting molecule. The all-electron results are very similar to previous results obtained using effective core potentials (ECP). A hybrid integration…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Charles W. Bauschlicher, , John W. Lawson

Asymmetric i/V curves with respect to the polarity of the voltage bias were observed in the Hg-Au junctions containing bilayers of alkanethiols of different chain length. Larger current resulted when a negative bias was applied to the metal…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Slawomir Sek , Marcin Majda

The variation of current I with voltage V for poly(phenylene vinylene) and other polymer light-emitting diodes has been attributed to carriers tunneling into broad conduction and valence bands. In actuality the electrons and holes tunnel…

Condensed Matter · Physics 2009-10-30 E. M. Conwell , M. W. Wu

We use a self-consistent method to study the distinct current-switch of $2^{'}$-amino-4-ethynylphenyl-4'-ethynylphenyl-5'-nitro-1-benzenethiol, from the first-principles calculations. The numerical results are in accord with the early…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 F. Jiang , Y. X. Zhou , H. Chen. R. Note , H. Mizuseki , Y. Kawazoe

In this work we consider a current carrying molecular junction with both electron-phonon and electron-electron interactions taken into account. After performing Lang-Firsov transformation and considering Markov approximations in accordance…

Mesoscale and Nanoscale Physics · Physics 2019-05-06 Amir Eskandari-asl

We investigate the origin of asymmetry in various measured current-voltage (I-V) characteristics of molecules with no inherent spatial asymmetry, with particular focus on a recent break junction measurement. We argue that such asymmetry…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Zahid , A. W. Ghosh , M. Paulsson , E. Polizzi , S. Datta

Conduction in pristine conjugated polymers (other than polyacetylene) is by polaron hopping between sites corresponding to conjugation lengths. The strong increase of current $I$ with voltage $V$ observed for both emission-limited and ohmic…

Soft Condensed Matter · Physics 2015-06-25 E. M. Conwell , M. W. Wu

The effect of substituting a hydrogen atom by a chlorine atom or a methyl group by a trichloromethyl (CCl3) group at the stereogenic center of light-driven second generation molecular motors is calculated in order to assess the effect on…

Chemical Physics · Physics 2025-10-10 Ivan Tambovtsev , Óskar Kristinsson , Hannes Jónsson

We consider exciton effects on current in molecular nanojunctions, using a model comprising a two two-level sites bridge connecting free electron reservoirs. Expanding the density operator in the many-electron eigenstates of the uncoupled…

Strongly Correlated Electrons · Physics 2015-05-14 GuangQi Li , Boris D. Fainberg , Abraham Nitzan , Sigmund Kohler , Peter Hänggi

The electronic transport through Au-(Cu$_{2}$O)$_n$-Au junctions is investigated using first-principles calculations and the nonequilibrium Green's function method. The effect of varying the thickness (i.e., $n$) is studied as well as that…

Materials Science · Physics 2016-06-07 Mohamed M. Fadlallah , Ulrich Eckern , Udo Schwingenschlögl

We measure the low bias conductance of a series of substituted benzene diamine molecules while breaking a gold point contact in a solution of the molecules. Transport through these substituted benzenes is by means of nonresonant tunneling…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Latha Venkataraman , Young S. Park , Adam C. Whalley Colin Nuckolls , Mark S. Hybertsen , Michael L. Steigerwald

The current-voltage ($I$-$V$) characteristics of break junctions of polycrystalline La$_{1.85}$Sr$_{0.15}$CuO$_4$, Y$_{0.75}$Lu$_{0.25}$Ba$_2$Cu$_3$O$_{7-\delta}$, Bi$_{1.8}$Pb$_{0.3}$Sr$_{1.9}$Ca$_2$Cu$_3$O$_x$ and composite…

Superconductivity · Physics 2007-11-22 D M Gokhfeld , D A Balaev , K A Shaykhutdinov , S I Popkov , M I Petrov

Current-voltage characteristics of Au~/~YBa$_2$Cu$_3$O$_{7-\delta}$ interfaces (Au/YBCO), built on optimally-doped YBCO thin films, grown by pulsed laser deposition, were measured as a function of temperature in the 50 K to 270 K range, for…

Materials Science · Physics 2020-02-19 L. F. Lanosa , H. Huhtinen , P. Paturi , C. Acha

Using a pi-orbital tight-binding model, we study the elastic and photoassisted transport properties of metal-molecule-metal junctions based on oligophenylenes of varying lengths. The effect of monochromatic light is modeled with an ac…

Mesoscale and Nanoscale Physics · Physics 2009-05-24 J. K. Viljas , F. Pauly , J. C. Cuevas

In this paper, we aim to understand the apparent characteristics of IQE and I-V curve in AlGaInP and InGaN LED devices. For the analysis, we separate the current into radiative current and non-radiative current component by using the…

Applied Physics · Physics 2017-05-29 Dong-Pyo Han , Jong-In Shim , Dong-Soo Shin

We investigate, by means of first-principles calculations, structural and transport properties of junctions made of symmetric dithiolated molecules placed between Au electrodes. As the electrodes are pulled apart, we find that it becomes…

Materials Science · Physics 2015-06-25 Ronaldo J. C. Batista , Pablo Ordejón , Hélio Chacham , Emilio Artacho

We have studied the influence of both exciton effects and Coulomb repulsion on current in molecular nanojunctions. We show that dipolar energy-transfer interactions between the sites in the wire can at high voltage compensate Coulomb…

Strongly Correlated Electrons · Physics 2012-01-16 Guangqi Li , Manmohan S. Shishodia , Boris D. Fainberg , Abraham Nitzan , Mark A. Ratner

We have carried out calculations of electron transport through a metal-molecule-metal junction with metal nanoclusters taking the part of electrodes. We show that negative differential resistance peaks could appear in the current-voltage…

Materials Science · Physics 2008-10-22 Natalya A. Zimbovskaya , Mark R. Pederson

The transport properties of a octane-dithiol (ODT) molecule coupled to Au(001) leads are analyzed using density functional theory and non-equilibrium Green functions. It is shown that a symmetric molecule can turn into a diode under…

Mesoscale and Nanoscale Physics · Physics 2010-02-09 Tomasz Kostyrko , Víctor M. García-Suárez , Colin J. Lambert , Bogdan R. Bułka

We have measured conductance histograms of atomic point contacts made from the noble-transition metal alloys CuNi, AgPd, and AuPt for a concentration ratio of 1:1. For all alloys these histograms at low bias voltage (below 300 mV) resemble…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Jan W. T. Heemskerk , Yves Noat , David J. Bakker , Jan M. van Ruitenbeek , Barend J. Thijsse , Peter Klaver
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