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We demonstrate direct time-domain observation of l-doubling contributions in molecular rotational dynamics using shaped femtosecond laser pulses. By imposing a tailored spectral phase on the excitation pulse, we pre-compensate centrifugal…

Quantum Physics · Physics 2026-05-05 Inbar Sternbach , Kfir Rutman Moshe , Amit Beer , Soumitra Hazra , Sharly Fleischer

It is shown that when relativistically intense ultrashort laser pulses are reflected from the boundary of a plasma with a near-critical density, Doppler frequency shift leads to generation of intense radiation both in the high-frequency, up…

Plasma Physics · Physics 2023-02-03 Nikita A. Mikheytsev , Artem V. Korzhimanov

The coherent interband dynamics of optically excited two-dimensional lateral surface superlattices driven by an in-plane static electric field has been investigated. The linear absorption, the spectrally-resolved pump-probe four-wave mixing…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 W. Yan , F. Claro , Z. Y. Zeng , Y. L. Zhao , J. Q. Liang

We present quantum mechanical explanations for unresolved phenomena observed in field-free molecular alignment by a femtosecond laser pulse. Quantum phase analysis of molecular rotational states reveals the physical origin of the following…

Optics · Physics 2015-04-09 Sang Jae Yun , Chul Min Kim , Jongmin Lee , Chang Hee Nam

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

We experimentally demonstrate generation of strong narrow-bandwidth emissions with excellent coherent properties at ~391 nm and ~428 nm from molecular ions of nitrogen inside a femtosecond filament in air by an orthogonally polarized…

The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…

Chemical Physics · Physics 2017-02-08 W. A. Bryan , C. R. Calvert , R. B. King , J. B. Greenwood , W. R. Newell , I. D. Williams

We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…

Atomic Physics · Physics 2018-04-03 Ruihua Xu , Zhaoyan Zhou , Xu Wang

We investigate bulk ion heating in solid buried layer targets irradiated by ultra-short laser pulses of relativistic intensities using particle-in-cell simulations. Our study focuses on a CD2-Al-CD2 sandwich target geometry. We find…

Plasma Physics · Physics 2013-10-22 Lingen Huang , Michael Bussmann , Thomas Kluge , Anle Lei , Wei Yu , Thomas E. Cowan

We consider the nonlinear propagation of electrostatic wave packets in an ultra-relativistic (UR) degenerate dense electron-ion plasma, whose dynamics is governed by the nonlocal two-dimensional nonlinear Schr{\"o}dinger-like equations. The…

Plasma Physics · Physics 2015-03-17 A. P. Misra , P. K. Shukla

We consider the classical dynamics of a two-electron system subjected to an intense bichromatic linearly polarized laser pulse. By varying the parameters of the field, such as the phase lag and the relative amplitude between the two colors…

Chaotic Dynamics · Physics 2011-04-04 Adam Kamor , Francois Mauger , Cristel Chandre , Turgay Uzer

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

It is shown that an undesirable curvature of the wave front of two-dimensional nonlinear wake wave excited in uniform plasma by a relativistic charged bunch or laser pulse may be compensated by radial change of the equilibrium plasma…

Plasma Physics · Physics 2009-11-06 A. G. Khachatryan

We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…

Atomic Physics · Physics 2016-08-24 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

The axial dependence of femtosecond filamentation in air is measured under conditions of varying laser pulsewidth, energy, and focusing f-number. Filaments are characterized by the ultrafast z-dependent absorption of energy from the laser…

High-order harmonic generation (HHG) in the relativistic regime is employed to obtain zeptosecond pulses of $\gamma$-rays. The harmonics are generated from atomic systems in counterpropagating strong attosecond laser pulse trains of linear…

Atomic Physics · Physics 2007-07-20 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We demonstrate that the THz generation in air from a dual-color pulse, composed of the fundamental and second-harmonic waves, can be coherently controlled by field-free molecular alignment. By tuning its time delay to properly match various…

Optics · Physics 2015-05-19 Jian Wu , Yuqi Tong , Min Li , Haifeng Pan , Heping Zeng

In standard lasers, light amplification requires population inversion between an upper and a lower state to break the reciprocity between absorption and stimulated emission. However, in a medium prepared in a specific superposition state,…

We investigate, through simulation, the evolution of polarization states during atmospheric propagation of high power, ultrashort laser pulses. A delayed rotational response model handling arbitrary, transverse polarization couples both the…

Optics · Physics 2015-06-16 J. P. Palastro

The time evolution of a two-level atom which is simultaneously exposed to the field of a running laser wave and a homogeneous gravitational field is studied. The result of the coupled dynamics of internal transitions and center-of-mass…

Quantum Physics · Physics 2016-09-08 Karl-Peter Marzlin , Juergen Audretsch