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We study the stability and structure of self-assembled atomic chains on Si(111) induced by monovalent, divalent and trivalent adsorbates, using first-principles total-energy calculations and scanning tunneling microscopy. We find that only…

Other Condensed Matter · Physics 2008-09-05 Corsin Battaglia , Philipp Aebi , Steven C. Erwin

The atomic structure of self-assembled quasi-one-dimensional Gd chains on Si(111) has been investigated by low-energy electron diffraction and scanning tunneling microscopy. Based on comparison between Gd and Ca chains we show that this Gd…

Other Condensed Matter · Physics 2007-05-23 C. Battaglia , H. Cercellier , C. Monney , M. G. Garnier , P. Aebi

Mn has been found to self-assemble into atomic chains running perpendicular to the surface dimer reconstruction on Si(001). They differ from other atomic chains by a striking asymmetric appearance in filled state scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2015-12-23 R. Villarreal , M. Longobardi , S. A. Köster , Ch. J. Kirkham , D. Bowler , Ch. Renner

Silica or SiO$_2$, the main constituent of earth's rocks has several 3D complex crystalline and amorphous phases, but it does not have a graphite like layered structure in 3D. Our theoretical analysis and numerical calculations from the…

Mesoscale and Nanoscale Physics · Physics 2014-06-24 V. Ongun Özçelik , S. Cahangirov , S. Ciraci

We report results on the self-assembly of silicon nanoribbons on the (2x1) reconstructed Au(110) surface under ultra-high vacuum conditions. Upon adsorption of 0.2 monolayer (ML) of silicon the (2x1) reconstruction of Au(110) is replaced by…

First-principles electronic-structure methods are used to study a structural model for Ag/Si(111)3x1 recently proposed on the basis of transmission electron diffraction data. The fully relaxed geometry for this model is far more…

Materials Science · Physics 2009-10-31 Steven C. Erwin , Hanno H. Weitering

The deposition of one silicon monolayer on Ag(111) gives rise to a set of superstructures depending on growth conditions. These superstructures are correlated to the epitaxy between the honeycomb structure of silicon (so called silicene)…

Materials Science · Physics 2015-09-30 H. Jamgotchian , B. Ealet , Y. Colignon , H. Maradj , J-Y. Hoarau , J-P. Biberian , B. Aufray

Monolayer structures made up of purely one kind of atoms are fascinating. Many kinds of honeycomb systems including carbon, silicon, germanium, tin, phosphorus and arsenic have been shown to be stable. However, so far the structures are…

Mesoscale and Nanoscale Physics · Physics 2015-08-25 C. Kamal , Aparna Chakrabarti , Motohiko Ezawa

Based on first-principles calculations of structure optimization, phonon modes and finite temperature molecular dynamics, we predict that silicon and germanium have stable, two-dimensional, low-buckled, honeycomb structures. Similar to…

Materials Science · Physics 2010-05-20 Seymur Cahangirov , Mehmet Topsakal , Ethem Akturk , Hasan Sahin , Salim Ciraci

Si(331)-(12x1) is the only confirmed planar silicon surface with a stable reconstruction located between (111) and (110). We have optimized the annealing sequence and are able to obtain almost defect free, atomically precise surface areas…

A new structural model for the Si(111)5x2-Au reconstruction is proposed and analyzed using first-principles calculations. The basic model consists of a "double honeycomb chain" decorated by Si adatoms. The 5x1 periodicity of the honeycomb…

Condensed Matter · Physics 2009-11-10 Steven C. Erwin

We report the first principle theory-based study of stability, electronic structure and optical properties of cluster assembled materials in various 1D, 2D and 3D nanostructures using a cage-like Cd9Te9 cluster as the super-atom. The bulk…

Mesoscale and Nanoscale Physics · Physics 2022-05-27 Kashinath T Chavan , Sharat Chandra

We present a first-principles study of bare and hydrogen passivated armchair nanoribbons of the puckered single layer honeycomb structures of silicon and germanium. Our study includes optimization of atomic structure, stability analysis…

Mesoscale and Nanoscale Physics · Physics 2010-12-21 S. Cahangirov , M. Topsakal , S. Ciraci

In the search for evidence of silicene, a two-dimensional honeycomb lattice of silicon, it is important to obtain a complete picture for the evolution of Si structures on Ag(111), which is believed to be the most suitable substrate for…

Materials Science · Physics 2015-06-04 Baojie Feng , Zijing Ding , Sheng Meng , Yugui Yao , Xiaoyue He , Peng Cheng , Lan Chen , Kehui Wu

Stress resulting from mismatch between a substrate and an adsorbed material has often been thought to be the driving force for the self-assembly of nanoscale structures. Bi nanolines self-assemble on Si(001), and are remarkable for their…

Materials Science · Physics 2009-11-07 J. H. G. Owen , K. Miki , H. Koh , H. W. Yeom , D. R. Bowler

The growth of the $\sqrt{3} \times \sqrt{3}$ reconstructed silicene on Ag substrate has been frequently observed in experiments while its atomic structure and formation mechanism is poorly understood. Here by first-principles calculations…

Mesoscale and Nanoscale Physics · Physics 2014-07-31 Seymur Cahangirov , Veli Ongun Özçelik , Lede Xian , Jose Avila , Suyeon Cho , María C. Asensio , Salim Ciraci , Angel Rubio

Possibility for the formation of stable Al atomic wire on the Si(211) surface is investigated using density functional theory based total energy calculations. The stable adsorption sites and the surface structures at various sub-monolayer…

Materials Science · Physics 2007-05-23 Bikash C Gupta , Inder P Batra

A new silicene-like family of reconstructed surfaces on Si111 are discussed which appears to be a polymorph to the well know family of surface reconstructions best epitomized by the 7x7 surface. Several experimental features are discussed…

Materials Science · Physics 2020-02-27 J. E. Demuth

We have carried out an ab-initio study of $\alpha$-Sn (111), with the aim of predicting and understanding its structure, reconstructions, and electronic states. We consider a variety of structural possibilities, and optimize them by moving…

Condensed Matter · Physics 2009-10-28 Zhong-Yi Lu , Guido L. Chiarotti , S. Scandolo , E. Tosatti

It is a well-established fact that the physical properties of compounds follow their crystal symmetries. This has especially pronounced implications on emergent collective quantum states in materials. Specifically, the effect of crystal…

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