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Microwave measurements have recently been successfully applied to measure ferroelectric materials on the nanoscale, including detection of polarization switching and ferroelectric domain walls. Here we discuss the question whether scanning…

Materials Science · Physics 2021-11-24 Mykola Yelisieiev , Petro Maksymovych , Anna N. Morozovska

Dielectric tensor and lattice dynamics of alpha-PbO2-type TiO2 have been investigated using the density functional perturbation theory, with a focus on responses of the vibrational frequencies to pressure. The calculated Raman spectra under…

Materials Science · Physics 2011-09-27 Yongqing Cai , Chun Zhang , Yuan Ping Feng

Hexagonal YMnO$_3$ is well known for the co-occurrence of ferroelectricity and antiferromagnetism at low temperatures. Using temperature-dependent spectroscopic ellipsometry at an $a$-plane oriented single crystal, we show how the…

Materials Science · Physics 2015-03-16 Steffen Richter , Stefan G. Ebbinghaus , Marius Grundmann , Rüdiger Schmidt-Grund

Temperature dependence of longitudinal optical phonons with oxygen character was measured in La1-xSrxMnO3 (x=0.2, 0.3) by inelastic neutron scattering in the (1 0 0) cubic direction. The zone center mode intensity is consistent with the…

Strongly Correlated Electrons · Physics 2007-05-23 D. Reznik , W. Reichardt

The origin of the low-temperature ferromagnetic instability in YTiO3 driven by the interplay between lattice, orbital, spin, and charge degrees of freedom is on the background of lattice dynamics. We present a comprehensive study of…

Strongly Correlated Electrons · Physics 2022-02-16 N. N. Kovaleva , O. E. Kusmartseva , A. Maljuk

We report detailed temperature-dependent inelastic neutron scattering and ab-initio lattice dynamics investigation of magnetic perovskites YCrO3 and LaCrO3. The magnetic neutron scattering from the Cr ions exhibits significant changes with…

Ilmenite-type crystals find a variety of technological applications due to their intriguing physical properties. We present the results of the lattice dynamics studies of honeycomb antiferromagnetic ilmenite CoTiO$_3$ single crystal by the…

Low-loss crystals with defects due to paramagnetic or rare earth impurity ions is a major area of investigation for quantum hybrid systems at both optical and microwave frequencies. In this work we examine the single crystal yttrium…

Materials Science · Physics 2017-08-02 N. C. Carvalho , M. Goryachev , J. Krupka , P. Bushev , M. E. Tobar

We present evidence for a concomitant structural and ferroelectric transformation around $T_S\sim 360$ K in multiferroic BiFeO$_3$/LaAlO$_3$ thin films close to the tetragonal phase. Phonon excitations are investigated by using Raman…

Strongly Correlated Electrons · Physics 2015-05-30 K. -Y. Choi , S. H. Do , P. Lemmens , D. Wulferding , C. S. Woo , J. H. Lee , K. Chu , C. -H. Yang

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

The dielectric properties of strontium titanate (SrTiO$_3$) have previously been reported from room temperature to low temperatures with conflicting results. In this work, precision measurement of the permittivity is undertaken by…

Materials Science · Physics 2015-09-01 Maxim Goryachev , Lingfei Zhao , Zijun Zhao , Warrick G. Farr , Jerzy Krupka , Michael E. Tobar

We report a study on the thermal conductivity (\kappa) of Tb_2Ti_2O_7 single crystals at low temperatures. It is found that in zero field this material has an extremely low phonon thermal conductivity in a broad temperature range. The mean…

Strongly Correlated Electrons · Physics 2013-06-11 Q. J. Li , Z. Y. Zhao , C. Fan , F. B. Zhang , H. D. Zhou , X. Zhao , X. F. Sun

Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…

Strongly Correlated Electrons · Physics 2015-10-28 C. Ulrich , G. Khaliullin , M. Guennou , H. Roth , T. Lorenz , B. Keimer

We revealed the anomalous temperature behavior of the giant dielectric permittivity and unusual frequency dependences of the pyroelectric response of the fine-grained ceramics prepared by the spark plasma sintering of the ferroelectric…

Phonon measurements in the A15-type superconductors were complicated in the past because of the unavailability of large single crystals for inelastic neutron scattering, e.g., in the case of Nb$_3$Sn, or unfavorable neutron scattering…

Superconductivity · Physics 2019-04-19 A. Sauer , D. A. Zocco , A. H. Said , R. Heid , A. Böhmer , F. Weber

We report inelastic neutron scattering measurements of the phonon spectra in a pure powder sample of the multiferroic material BiFeO3. A high-temperature range was covered to unravel the changes in the phonon dynamics across the Neel (T_N ~…

Materials Science · Physics 2015-03-19 M. Zbiri , H. Schober , N. Choudhury , R. Mittal , S. L. Chaplot , S. J. Patwe , S. N. Achary , A. K. Tyagi

We investigate single crystals of the trigonal antiferromagnet EuZn$_2$P$_2$ ($P\overline{3}m1$) by means of electrical transport, magnetization measurements, X-ray magnetic scattering, optical reflectivity, angle-resolved photoemission…

We have carried out temperature-dependent x-ray diffraction and Raman scattering experiments on powder $Cs_3Bi_2Br_9$. Trigonal to monoclinic structural transition at around 95 K is discussed and shown to be driven by the softening of the…

The phase purity and the lattice dynamics in bulk EuTiO3 were investigated both microscopically, using X-ray and neutron diffraction, 151-Eu-M\"ossbauer spectroscopy, and 151-Eu nuclear inelastic scattering, and macroscopically using…

Strongly Correlated Electrons · Physics 2013-10-30 D. Bessas , K. Z. Rushchanskii , M. Kachlik , S. Disch , O. Gourdon , J. Bednarcik , K. Maca , I. Sergueev , S. Kamba , M. Ležaíc , R. P. Hermann

We have studied the optical properties of the heavy-fermion compound UNi2Al3 at frequencies between 100 GHz and 1 THz (3 cm^-1 and 35 cm^-1), temperatures between 2 K and 300 K, and magnetic fields up to 7 T. From the measured transmission…

Strongly Correlated Electrons · Physics 2012-11-14 Julia P. Ostertag , Marc Scheffler , Martin Dressel , Martin Jourdan