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We address the response of a random heteropolymer to preferential solvation of certain monomer types at the globule-solvent interface. For each set of monomers that can comprise the molecule's surface, we represent the ensemble of allowed…

Soft Condensed Matter · Physics 2009-11-10 Philip Geissler , Eugene Shakhnovich , Alexander Grosberg

We study clogging of cohesive particles in a 2D hopper with experiments and simulations. The system consists of buoyant, monodisperse oil droplets in an aqueous solution, where the droplet size, buoyant force, cohesion, and hopper opening…

Soft Condensed Matter · Physics 2026-02-26 Johnathan Hoggarth , Pablo E. Illing , Eric R. Weeks , Kari Dalnoki-Veress

Given the wide range of length scales, the analysis of polymer systems often requires coarse-graining, for which various levels of description may be possible depending on the phenomenon under consideration. Here, we provide a super-coarse…

Soft Condensed Matter · Physics 2024-09-05 Naoki Iso , Yuki Norizoe , Takahiro Sakaue

We present numerical calculations of lamellar phases of block copolymers at patterned surfaces. We model symmetric di-block copolymer films forming lamellar phases and the effect of geometrical and chemical surface patterning on the…

Soft Condensed Matter · Physics 2016-02-18 Xingkun Man , David Andelman , Henri Orland

We study a d-dimensional lattice model of diffusing coalescing massive particles, with two parameters controlling deposition and evaporation of monomers. The unique stationary distribution for the system exhibits a phase transition in all…

Probability · Mathematics 2016-08-09 Colm Connaughton , R. Rajesh , Roger Tribe , Oleg Zaboronski

We study a mutually coupled mesoscopic-macroscopic-shell system of equations modeling a dilute incompressible polymer fluid which is evolving and interacting with a flexible shell of Koiter type. The polymer constitutes a solvent-solute…

Analysis of PDEs · Mathematics 2021-03-17 Dominic Breit , Prince Romeo Mensah

By means of extensive Monte Carlo simulations of the bond fluctuation model, we study the effect of adding AB diblock copolymers on the properties of an interface between demixed homopolymer phases. The parameters are chosen such that the…

Soft Condensed Matter · Physics 2009-10-31 A. Werner , F. Schmid , M. Mueller

We use computer simulations to study the relaxation dynamics of a model for oil-in-water microemulsion droplets linked with telechelic polymers. This system exhibits both gel and glass phases and we show that the competition between these…

Soft Condensed Matter · Physics 2015-05-29 Pinaki Chaudhuri , Pablo I. Hurtado , Ludovic Berthier , Walter Kob

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

Statistical Mechanics · Physics 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov

A coarse-grained model for solutions of polymers in supercritical fluids is introduced and applied to the system of hexadecane and carbon dioxide as a representative example. Fitting parameters of the model to the gas-liquid critical point…

Soft Condensed Matter · Physics 2009-11-10 P. Virnau , M. Mueller , L. G. MacDowell , K. Binder

We have studied the phase behavior of the poly(n-butyl acrylate)-b-poly(acrylic acid) block copolymer in a mixture of two miscible solvents, water and tetrahydrofuran (THF). The techniques used to examine the different polymers, structures…

We derive a mode-coupling theory for the slow dynamics of fluids confined in disordered porous media represented by spherical particles randomly placed in space. Its equations display the usual nonlinear structure met in this theoretical…

Soft Condensed Matter · Physics 2007-05-23 V. Krakoviack

Letting free polymers diffuse from solution into a crosslinked polymer gel is often a crucial processing step in the synthesis of multiphase polymer-based gels, e.g., core-shell microgels. Here we use coarse-grained molecular dynamics…

Soft Condensed Matter · Physics 2024-12-17 Jude Ann Vishnu , Torsten Gereon Linder , Sebastian Seiffert , Friederike Schmid

We study the diffusion of a linear polymer in the presence of permeable membranes without excluded volume interactions, using scaling theory and Monte Carlo simulations. We find that the average time it takes for a chain with polymerization…

Condensed Matter · Physics 2016-08-31 Hyoungsoo Yoon , J. M. Deutsch

Conformational phases of a semiflexible off-lattice homopolymer model near an attractive substrate are investigated by means of multicanonical computer simulations. In our polymer-substrate model, nonbonded pairs of monomers as well as…

Computational Physics · Physics 2009-07-20 Monika Möddel , Michael Bachmann , Wolfhard Janke

The self-assembly of copolymeric vesicles and micelles in micromixers is studied by External Potential Dynamics (EPD) simulations -- a dynamic density functional approach that explicitly accounts for the polymer architecture both at the…

Soft Condensed Matter · Physics 2018-04-10 Simon Kessler , Klaus Drese , Friederike Schmid

We present a theoretical model for predicting the phase behavior of polymer solutions in which phase separation competes with oligomerization. Specifically, we consider scenarios in which the assembly of polymer chains into stoichiometric…

Soft Condensed Matter · Physics 2024-07-31 Tianhao Li , W. Benjamin Rogers , William M. Jacobs

Using molecular dynamic simulations we study a waterlike model confined between two fixed hydrophobic plates. The system is tested for density, diffusion and structural anomalous behavior and compared with the bulk results. Within the range…

Chemical Physics · Physics 2013-03-06 Leandro Batirolla Krott , Marcia Cristina Bernardes Barbosa

The coagulation of dust aggregates occurs in various astrophysical environments. Each one is characterized by different conditions that influence the growth, e.g. relative velocities, composition, and size of the smallest constituents…

Solar and Stellar Astrophysics · Physics 2015-05-14 D. Paszun , C. Dominik

We present an extensive numerical study of the critical behavior of dimer models in three dimensions, focusing on the phase transition between Coulomb and crystalline columnar phases. The case of attractive interactions between parallel…

Strongly Correlated Electrons · Physics 2015-03-17 D. Charrier , F. Alet