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The Mott-insulator \kappa-(BEDT-TTF)_2Cu_2(CN)_3 is the prime candidate of a quantum spin liquid with puzzling magnetic properties. Our THz and infrared investigations reveal that also the charge dynamics does not follow the expectations…

Strongly Correlated Electrons · Physics 2012-11-06 Sebastian Elsasser , Dan Wu , Martin Dressel , John A. Schlueter

The electrodynamic response of the organic spin-liquid candidate $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been measured in an extremely wide energy range ($10^{-13}$ to 2 eV) as a function of temperature (5 to 300 K). Below the Mott gap,…

Strongly Correlated Electrons · Physics 2014-12-16 A. Pustogow , E. Zhukova , B. Gorshunov , M. Pinterić , S. Tomić , J. A. Schlueter , M. Dressel

In this paper we study the optical properties of $U(1)$ spin liquids with large spinon Fermi surfaces based on a simple formula for the bulk optical conductivity obtained through the Ioffe-Larkin composition rule. We show that the optical…

Strongly Correlated Electrons · Physics 2015-03-20 Yuan-Fei Ma , Tai-Kai Ng

Recent terahertz conductivity measurements observed low-power-law frequency dependence of optical conduction within the Mott gap of the Kagome lattice spin-liquid candidate Herbertsmithite. We investigate mechanisms for this observed…

Strongly Correlated Electrons · Physics 2013-06-12 Andrew C. Potter , T. Senthil , Patrick A. Lee

We show that the optical spin conductivity being a small AC response of a bulk spin current and elusive in condensed matter systems can be measured in ultracold atoms. We demonstrate that this conductivity contains rich information on…

Quantum Gases · Physics 2022-10-14 Yuta Sekino , Hiroyuki Tajima , Shun Uchino

The quest for entangled spin excitations has stimulated intense research on frustrated magnetic systems. For almost two decades, the triangular-lattice Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been the hottest candidate for…

Strongly Correlated Electrons · Physics 2023-06-06 A. Pustogow , Y. Kawasugi , H. Sakurakoji , N. Tajima

We numerically investigate the dynamical properties of $\kappa$-type molecular conductors in their antiferromagnetic Mott insulating state. By treating the extended Hubbard model on the two-dimensional $\kappa$-type lattice within the…

Strongly Correlated Electrons · Physics 2021-06-22 Hitoshi Seo , Makoto Naka

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…

We investigate the continuous variation of electronic states from a Fermi liquid to a quantum spin liquid induced by chemical substitution in the organic dimer-Mott system of $\kappa$-[(BEDSe-TTF)$_x$(BEDT-TTF)$_{1-x}$]$_2$Cu[N(CN)$_2$]Br.…

Strongly Correlated Electrons · Physics 2022-04-06 Shusaku Imajo , Naoko Kato , Robert J. Marckwardt , Emre Yesil , Hiroki Akutsu , Yasuhiro Nakazawa

It has been more than 40 years since superconductivity was discovered in organic conductors, and the way scientists view organic superconductors has changed over time. At first, the fact that organic conductors exhibit superconductivity was…

Superconductivity · Physics 2023-07-20 Hiroshi Oike , Hiromi Taniguchi , Kazuya Miyagawa , Kazushi Kanoda

The coupling of the spin of electrons to their motional state lies at the heart of recently discovered topological phases of matter. Here we create and detect spin-orbit coupling in an atomic Fermi gas, a highly controllable form of quantum…

The properties of the pseudogap phase above Tc of the high-Tc cuprate superconductors are described by showing that the Anderson-Nambu SU(2) spinors of an RVB spin gap 'lock' to those of the electron charge system because of the resulting…

Superconductivity · Physics 2015-06-25 Philip Anderson

We study the theory of a U(1) gauge field coupled to a spinon Fermi surface. Recently this model has been proposed as a possible description of the organic compound $\kappa-(BEDT-TTF)_2 Cu_2 (CN)_3$. We calculate the susceptibility of this…

Strongly Correlated Electrons · Physics 2009-11-11 Cody P. Nave , Sung-Sik Lee , Patrick A. Lee

The dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ exhibits unusual electrodynamic properties. Numerical investigations of the electronic ground state and the molecular and lattice vibrations reveal the importance of the…

Strongly Correlated Electrons · Physics 2016-02-02 M. Dressel , P. Lazic , A. Pustogow , E. Zhukova , B. Gorshunov , J. A. Schlueter , O. Milat , B. Gumhalter , S. Tomic

Recent studies of organic molecular solids are highlighted by their complex phase diagram and light-induced phenomena, such as Mott insulator, spin liquid phase, and superconductivity. However, a discrepancy between experimental observation…

Strongly Correlated Electrons · Physics 2024-12-25 Dongbin Shin , Fabijan Pavošević , Nicolas Tancogne-Dejean , Michele Buzzi , Emil Viñas Boström , Angel Rubio

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

Strongly Correlated Electrons · Physics 2018-05-01 Martin Dressel , Andrej Pustogow

In this paper we study the nonlinear current response of $U(1)$ spin liquids with large spinon Fermi surfaces under the perturbation of a time-dependent ac electric field $\mathbf{E}(t)$ within the framework of an effective $U(1)$ gauge…

Strongly Correlated Electrons · Physics 2016-06-15 Yuan-Fei Ma , Tai-Kai Ng

Fermi liquid theory is remarkably successful in describing the transport and optical properties of metals; at frequencies higher than the scattering rate, the optical conductivity adopts the well-known power law behavior $\sigma_1(\omega)…

Superconductivity · Physics 2013-12-17 C. C. Homes , J. J. Tu , J. Li , G. D. Gu , A. Akrap

Recent experiments on the organic compound $\kappa-(BEDT-TTF)_2 Cu_2 (CN)_3$ raise the possibility that the system may be described as a quantum spin liquid. Here we propose a pairing state caused by the `Amperean' attractive interaction…

Strongly Correlated Electrons · Physics 2007-05-23 Sung-Sik Lee , Patrick A. Lee , T. Senthil

A low energy crossover (see cond-mat/9711167) induced by Fermi liquid reservoirs in transport through a 1D Mott-Hubbard insulator of finite length $L$ is examined in the presence of impurity pinning. Under the assumption that the Hubbard…

Condensed Matter · Physics 2009-10-31 Vadim Ponomarenko , Naoto Nagaosa
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