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We propose schemes to produce highly nuclear-spin polarized small molecules in an intense and cold molecular beam via microwave or infrared rotational excitation, followed by hyperfine-induced quantum beats. Repumping schemes can be used to…

Chemical Physics · Physics 2026-03-20 C. S. Kannis , T. P. Rakitzis

We demonstrate that the dynamic nuclear polarization (DNP) of phosphorus donors in silicon can be very effective in a magnetic field of 4.6 T and at temperatures below 1 K. The DNP occurs due to the Overhauser effect following a cross…

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle…

We propose a correction to the coefficient of nuclear-spin diffusion by a factor $1/\sqrt{1-\overline{p}^{2}}$, where $\overline{p}$ is the average nuclear-spin polarization. The correction, derived by extending the Lowe-Gade theory to…

Other Condensed Matter · Physics 2021-06-25 Yu Wang , Kazuyuki Takeda

An efficient technique to generate ensembles of spins that are highly polarized by external magnetic fields is the Holy Grail in Nuclear Magnetic Resonance (NMR) spectroscopy. Since spin-half nuclei have steady-state polarization biases…

Quantum Physics · Physics 2007-05-23 Jose M. Fernandez , Seth Lloyd , Tal Mor , Vwani Roychowdhury

We report a large enhancement of 1.7 in deuteron polarization up to values of 0.6 due to frequency modulation of the polarizing microwaves in a two liters polarized target using the method of dynamic nuclear polarization. This target was…

High Energy Physics - Experiment · Physics 2012-08-27 The SMC Collaboration

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

The spin diffusion and damped oscillations are studied in the collision of two spin polarized clouds of cold atoms with resonant interactions. The strong density dependence of the diffusion coefficient leads to inhomogeneous spin diffusion…

Quantum Gases · Physics 2015-06-03 H. Heiselberg

A new method for local dynamic nuclear polarization is demonstrated in a GaAs/AlGaAs heterostructure at the Landau level filling factor $\nu=3$. Using a narrow channel sample, where the width varies stepwise along the electron flow, we find…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yosuke Komori , Tohru Okamoto

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

Physical systems reach thermal equilibrium through energy exchange with their environment, and for spins in solids the relevant environment is almost always the host lattice in which they sit. However, recent studies motivated by…

Dynamic nuclear polarization (DNP) can increase nuclear magnetic resonance (NMR) signals by orders of magnitude. DNP in diamond proceeds through different DNP mechanisms with a possible temperature-dependence. We report on 13C dynamic…

Rapid injection of spin polarization into an ensemble of nuclear spins is a problem of broad interest, spanning dynamic nuclear polarization (DNP) to quantum information science. We report on a strategy to boost the spin injection rate by…

We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy…

Quantum Physics · Physics 2013-04-01 Ran Fischer , Andrey Jarmola , Pauli Kehayias , Dmitry Budker

There has been much recent research into polarizing an antiproton beam, instigated by the recent proposal from the PAX (Polarized Antiproton eXperiment) project at GSI Darmstadt. It plans to polarize an antiproton beam by repeated…

High Energy Physics - Phenomenology · Physics 2008-11-26 N. H. Buttimore , D. S. O'Brien

We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling…

Mesoscale and Nanoscale Physics · Physics 2013-02-13 V. Ranjan , G. de Lange , R. Schutjens , T. Debelhoir , J. P. Groen , D. Szombati , D. J. Thoen , T. M. Klapwijk , R. Hanson , L. DiCarlo

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

A dynamical nuclear polarization scheme is studied in gated double dots. We demonstrate that a small polarization ($\sim 0.5%$) is sufficient to enhance the singlet decay time by two orders of magnitude. This enhancement is attributed to an…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Guy Ramon , Xuedong Hu

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…

Quantum Physics · Physics 2023-04-10 Timur V. Tscherbul , Jun Ye , Ana Maria Rey

We investigate analytically and numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the dipolar ordered initial state. We suggest two different methods…

Other Condensed Matter · Physics 2009-11-13 S. I. Doronin , E. B. Fel'dman , E. I. Kuznetsova , G. B. Furman , S. D. Goren