Related papers: Photon Statistics for Single Molecule Non-Linear S…
We investigate the possibility of measuring the homogeneous and inhomogeneous contribution to the linewidth of a spectrally diffusing single photon emitter using a simple photon correlation spectroscopy method (PCS). The photon energy…
For the first time a method for realizing macroscopic quantum optical solitons is presented. Simultaneous photon-number and momentum squeezing is predicted using soliton propagation in an interferometer. Extraction of soliton pulses closer…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
Non-classical correlations in optical beams offer the unprecedented opportunity of surpassing conventional limits of sensitivity and resolution in optical measurements and imaging, especially but not only, when a low photon flux down to the…
In this paper, we present a novel stochastic and spatially lumped multi-mode model to describe the nonlinear dynamics of actively Q-switched lasers and random perturbations due to amplified spontaneous emission. This model will serve as a…
In a single-particle detection experiment, a wavefront impinges on a detector but observers only see a point response. The extent of the wavefront becomes evident only in statistical accumulation of many independent detections, with…
We present a detailed overview of the physics of two-color soliton molecules in nonlinear waveguides, i.e. bound states of localized optical pulses which are held together due to an incoherent interaction mechanism. The mutual confinement,…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…
Spontaneous emission (SE) from a two-level atom in a photonic crystal (PC) with anisotropic one-band model is investigated using the fractional calculus. Analytically solving the kinetic equation in terms of the fractional exponential…
We investigate the photon statistics of an ensemble of coherently driven non-interacting two-level atoms in the weak driving regime. As it turns out, the system displays unique emission characteristics that are strongly in contrast to the…
We derive the statistical limit of the spectral autocorrelation function and of the survival probability for the indirect photodissociation of molecules in the regime of non-overlapping resonances. The results are derived in the framework…
We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…
Photon statistics is a powerful tool for characterizing the emission dynamics of nanoscopic systems and their photophysics. Recent advances that combine correlation spectroscopy with scanning tunneling microscopy-induced luminescence (STML)…
Nonlinear spectroscopy is widely used to study the transient dynamics of molecules under strong light-matter coupling, though it remains unclear to what extent uncoupled intracavity molecules obscure signals from the strongly-coupled…
In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…
Molecular electronics is a rapidly developing field focused on using molecules as the structural basis for electronic components. It is common in such devices for the system of interest to couple simultaneously to multiple environments.…
A new type of artificial molecule is proposed, which consists of coupled defect atoms in photonic crystals, named as photonic molecule. Within the major band gap, the photonic molecule confines the resonant modes that are closely analogous…
This proposal investigates the photon-statistics of light emitted by a statistical ensemble of cold atoms excited by the near-field of an optical nanofiber tip. Dipole-dipole interactions of atoms at such short distance from each other…
Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…