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Using small-angle neutron scattering and liquid integral equation theory, we relate the structure factor of flexible dendrimers of 4th generation to their average shape. The shape is measured as a radial density profile of monomers…

Soft Condensed Matter · Physics 2009-10-31 C. N. Likos , M. Schmidt , H. Loewen , M. Ballauff , D. Poetschke , P. Lindner

A relationship between the measurable monomer-monomer structure factor, and the centre-of-mass (CM) structure factor of dilute or semi-dilute polymer solutions is derived from Ornstein-Zernike relations within the ``polymer reference…

Soft Condensed Matter · Physics 2009-11-07 V. Krakoviack , J. P. Hansen , A. A. Louis

We consider ring polymers in good solvents in the dilute limit. We determine the structure factor and the monomer-monomer distribution function. We compute accurately the asymptotic behavior of these functions for small and large momenta…

Statistical Mechanics · Physics 2009-11-07 Pasquale Calabrese , Andrea Pelissetto , Ettore Vicari

The dynamic structure factor of semiflexible polymers in solution is derived from the wormlike chain model. Special attention is paid to the rigid constraint of an inextensible contour and to the hydrodynamic interactions. For the cases of…

Soft Condensed Matter · Physics 2009-10-28 Klaus Kroy , Erwin Frey

Density functional theory for a simple model of dendrimers is proposed. The theory is based on fundamental measure theory which accounts for the hard-sphere repulsion of the segments and on the Wertheim first-order perturbation theory for…

Soft Condensed Matter · Physics 2012-11-12 Alexandr Malijevsky

As an important physical quantity to understand the internal structure of polymer chains, the structure factor is being studied both in theory and experiment. Theoretically, the structure factor of Gaussian chains have been solved…

Soft Condensed Matter · Physics 2021-04-21 Jie Huang , Xinghua Zhang , Gang Huang , Shiben Li

We study the influence of mutual interaction on the conformation of flexible poly(propyleneamine) dendrimers of fourth generation in concentrated solution. Mixtures of dendrimers with protonated and deuterated end groups are investigated by…

Soft Condensed Matter · Physics 2009-07-08 S. Rosenfeldt , M. Ballauff , P. Lindner , L. Harnau

We use the thread model for linear chains of interacting monomers, and the ``polymer reference interaction site model'' (PRISM) formalism to determine the monomer-monomer pair correlation function $h_{mm}(r)$ for dilute and semi-dilute…

Soft Condensed Matter · Physics 2007-05-23 V. Krakoviack , B. Rotenberg , J. -P. Hansen

Polymer reference interaction site model (PRISM) theory, a descendent of Ornstein-Zernike liquid state theory, is a powerful tool to predict the structure and thermodynamics of equilibrium polymer systems, but its accuracy and applicability…

Soft Condensed Matter · Physics 2025-11-19 Zhihao Feng , Christian T. Randolph , Tyler B. Martin , Thomas E. Gartner

We have studied the conformational and scaling behaviors of a flexible dendrimer immersed in athermal or good solvents. A self-consistent field theory combined with a pre-averaged excluded volume potential representing the two-body…

Soft Condensed Matter · Physics 2018-08-30 Meng Shi , Yingzi Yang , Feng Qiu

Entangled polymers are deformed by a strong shear flow. The shape of the polymer, called the form factor, is measured by small angle neutron scattering. However, the real-space molecular structure is not directly available from the…

We provide a comprehensive overview of the current theoretical understanding of the dynamic structure factor of stiff polymers in semidilute solution based on the wormlike chain (WLC) model. We extend previous work by computing exact…

Soft Condensed Matter · Physics 2008-05-29 J. Glaser , O. Hallatschek , K. Kroy

The structure of flexible polymers endgrafted in cylindrical pores of diameter D is studied as a function of chain length N and grafting density \sigma, assuming good solvent conditions. A phenomenological scaling theory, describing the…

Soft Condensed Matter · Physics 2009-11-11 D. I. Dimitrov , A. Milchev , K. Binder

Closed analytical expressions for scattering intensity and other global structure factors are derived for a new solvable model of polydisperse sticky hard spheres. The starting point is the exact solution of the ``mean spherical…

Statistical Mechanics · Physics 2009-10-31 Domenico Gazzillo , Achille Giacometti

We consider a system of particles interacting via a purely repulsive, soft-core potential recently introduced to model effective pair interactions between dendrimers, which is expected to lead to the formation of crystals with multiple…

Soft Condensed Matter · Physics 2015-05-11 Davide Pini

In this work, we consider a semi-dilute solution of identical star-polymers, made of attached flexible long polymer chains of the same polymerization degree N. We first compute the effective pair-potential between star-polymers. Such a…

Soft Condensed Matter · Physics 2007-05-23 F. Benzouine , M. Yassine , A. Derouiche , A. Bettachy , M. Benhamou

The effective pair potentials between different kinds of dendrimers in solution can be well approximated by appropriate Gaussian functions. We find that in binary dendrimer mixtures the range and strength of the effective interactions…

Soft Condensed Matter · Physics 2007-05-23 I. O. Gotze , A. J. Archer , C. N. Likos

We exemplarily investigate how optical properties of single scatterers in interacting multi-particle systems influence measurable structure factors. Both particles with linear gradients of their scattering length density and core-shell…

Soft Condensed Matter · Physics 2024-04-05 Joel Diaz Maier , Katharina Gaus , Joachim Wagner

Small-angle scattering is a commonly used tool to analyze the dispersion of nanoparticles in all kinds of matrices. Besides some obvious cases, the associated structure factor is often complex and cannot be reduced to a simple interparticle…

Soft Condensed Matter · Physics 2023-10-24 Anne-Caroline Genix , Julian Oberdisse

We study the optimal design of numerical integrators for dissipative systems, for which there exists an underlying thermodynamic structure known as GENERIC (general equation for the nonequilibrium reversible-irreversible coupling). We…

Numerical Analysis · Mathematics 2020-02-14 Xiaocheng Shang , Hans Christian Öttinger
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