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We present a molecular dynamics study of the effects of confinement on the lubrication and flow properties of ionic liquids. We use a coarse-grained salt model description of ionic liquid as a lubricant confined between finite solid plates…

Soft Condensed Matter · Physics 2018-11-08 Miljan Dašić , Konstantinos Gkagkas , Igor Stanković

The slip of a fluid layer in contact with a solid confining surface is investigated for different temperatures and densities using molecular dynamic simulations. We show that for an anomalous water-like fluid the slip goes as follows: for…

Soft Condensed Matter · Physics 2018-03-21 Patricia Ternes , Evy Salcedo , Marcia C. Barbosa

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer

We study the effects of confinement between two parallel walls on a two dimensional fluid with competing interactions which lead to the formation of particle micro-domains at the thermodynamic equilibrium (microphases or microseparation).…

Soft Condensed Matter · Physics 2009-11-13 A. Imperio , L. Reatto

The physics of diffusion phenomena in nano and micro channels has attracted a lot of attention in recent years, due to its close connection with many technological, medical and industrial applications. In the present paper we employ a…

Soft Condensed Matter · Physics 2015-09-30 Umberto Marini Bettolo Marconi , Paolo Malgaretti , Ignacio Pagonabarraga

A simple fluid, described by point-like particles interacting via the Lennard-Jones potential, is considered under confinement in a slit geometry between two walls at distance Lz apart for densities inside the vapor-liquid coexistence…

Soft Condensed Matter · Physics 2009-11-13 Katarzyna Bucior , Leonid Yelash , Kurt Binder

We extend the transfer matrix method of one-dimensional hard core fluids placed between confining walls for that case where the particles can pass each other and at most two layers can form. We derive an eigenvalue equation for a…

Statistical Mechanics · Physics 2015-06-29 Peter Gurin , Szabolcs Varga

We present mode-coupling theory (MCT) results for densely packed hard-sphere fluids confined between two parallel walls and compare them quantitatively to computer simulations. The numerical solution of MCT is calculated for the first time…

Soft Condensed Matter · Physics 2023-05-10 Gerhard Jung , Thomas Franosch

The complex behavior of confined fluids arising due to a competition between layering and local packing can be disentangled by considering quasi-confined liquids, where periodic boundary conditions along the confining direction restore…

Soft Condensed Matter · Physics 2020-09-03 Lukas Schrack , Charlotte F. Petersen , Gerhard Jung , Michele Caraglio , Thomas Franosch

Packing frustration for confined fluids, i.e., the incompatibility between the preferred packing of the fluid particles and the packing constraints imposed by the confining surfaces, is studied for a dense hard-sphere fluid confined between…

Soft Condensed Matter · Physics 2014-09-05 Kim Nygård , Sten Sarman , Roland Kjellander

We show using computer simulations and mean field theory that a system of particles in two dimensions, when confined laterally by a pair of parallel hard walls within a quasi one dimensional channel, possesses several anomalous structural…

Soft Condensed Matter · Physics 2009-11-13 Debasish Chaudhuri , Surajit Sengupta

The properties of nanoconfined fluids can be strikingly different from those of bulk liquids. A basic unanswered question is whether the equilibrium and dynamic consequences of confinement are related to each other in a simple way. We study…

Soft Condensed Matter · Physics 2013-12-17 Trond S. Ingebrigtsen , Jeffrey R. Errington , Thomas M. Truskett , Jeppe C. Dyre

Performing molecular dynamics simulations, we investigate the enormous slowdowns of water dynamics when approaching a glass transition or a solid interface. We show that both effects can be described on common grounds within a theoretical…

Soft Condensed Matter · Physics 2015-06-19 Felix Klameth , Michael Vogel

The collective diffusion of dense fluids in spatial confinement was studied by combining high-energy (21 keV) x-ray photon correlation spectroscopy and small-angle x-ray scattering from colloid-filled microfluidic channels. We found the…

Soft Condensed Matter · Physics 2016-05-04 Kim Nygard , Johan Buitenhuis , Matias Kagias , Konstantins Jefimovs , Federico Zontone , Yuriy Chushkin

The static and dynamical properties of heavy water have been studied at ambient conditions with extensive Car-Parrinello molecular-dynamics simulations in the canonical ensemble, with temperatures ranging between 325 K and 400 K.…

Soft Condensed Matter · Physics 2007-05-23 P. H-L. Sit , Nicola Marzari

When a fluid that undergoes a vapor to liquid transition in the bulk is confined to a long cylindrical pore, the phase transition is shifted (mostly due to surface effects at the walls of the pore) and rounded (due to finite size effects).…

Statistical Mechanics · Physics 2015-05-19 Alexander Winkler , Dorothea Wilms , Peter Virnau , Kurt Binder

We investigate theoretically and numerically the impact of an elastic sphere on a rigid wall in a viscous fluid. Our focus is on the dynamics of the contact, employing the soft lubrication model in which the sphere is separated from the…

Soft Condensed Matter · Physics 2024-05-08 Vincent Bertin

We report a molecular dynamics simulation investigating the dynamics of a simple liquid in the proximity to a non-interacting smooth confining wall. A strong enhancement of the liquid diffusion is observed within the layers adjacent to the…

Materials Science · Physics 2024-12-06 Lorenzo Agosta , Mikhail Dzugutov , Wim Briels , Kersti Hermansson

Recent discoveries have spurred the theoretical prediction and experimental realization of novel materials that have topological properties arising from band inversion. Such topological insulators are insulating in the bulk but have…

Mesoscale and Nanoscale Physics · Physics 2017-07-26 M. Kotulla , U. Zülicke

Fluctuations in a fluid are strongly affected by the presence of a macroscopic gradient making them long-ranged and enhancing their amplitude. While small-scale fluctuations exhibit diffusive lifetimes, larger-scale fluctuations live…