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A comparison of simulation results with the prediction of the structural properties of square-shoulder fluids is carried out to assess the performance of three theories: Tang--Lu's first-order mean spherical approximation, the simplified…

Soft Condensed Matter · Physics 2016-03-01 M. López de Haro , S. B. Yuste , A. Santos

Monte Carlo simulations on the structural properties of ternary fluid mixtures of additive hard spheres are reported. The results are compared with those obtained from a recent analytical approximation [S. B. Yuste, A. Santos, and M. Lopez…

Statistical Mechanics · Physics 2007-05-23 Alexander Malijevsky , Anatol Malijevsky , Santos B. Yuste , Andres Santos , Mariano Lopez de Haro

We discuss phase coexistence of polydisperse colloidal suspensions in the presence of adhesion forces. The combined effect of polydispersity and Baxter's sticky-hard-sphere (SHS) potential, describing hard spheres interacting via strong and…

Statistical Mechanics · Physics 2009-11-11 Domenico Gazzillo , Achille Giacometti , Riccardo Fantoni

Integral equation of pure liquids, combined with a new "scaling approximation" based on a corresponding states treatment of pair correlation functions, is used to evaluate approximate structure factors for colloidal fluids constituted of…

The chemical potential of a hard-sphere fluid can be expressed in terms of the contact value of the radial distribution function of a solute particle with a diameter varying from zero to that of the solvent particles. Exploiting the…

Statistical Mechanics · Physics 2012-09-24 Andrés Santos

In this work we extend the applicability of the microcanonical ensemble simulation method, originally proposed to study the Ising model (A. H\"uller and M. Pleimling, Int. Journal of Modern Physics C, 13, 947 (2002),…

Statistical Mechanics · Physics 2015-09-16 Francisco Sastre , Ana Laura Benavides , José Torres-Arenas , Alejandro Gil-Villegas

Certain models with purely repulsive pair interactions can form cluster crystals with multiply-occupied lattice sites. Simulating these models' equilibrium properties is, however, quite challenging. Here, we develop an expanded…

Soft Condensed Matter · Physics 2015-03-20 Kai Zhang , Patrick Charbonneau

The structural properties of fluids whose molecules interact via potentials with a hard-core plus n piece-wise constant sections of different widths and heights are derived using a (semi-analytical) rational-function approximation method.…

Soft Condensed Matter · Physics 2012-07-13 A. Santos , S. B. Yuste , M. López de Haro

Based on the path integral representation of the partition function of a many body system with separable two body interaction we propose a systematic extension of the perturbed static path approximation (PSPA) to lower temperatures.…

Statistical Mechanics · Physics 2009-11-07 Christian Rummel , Joachim Ankerhold

We study a fluid-fluid phase transition of the explicit solvent model represented as a mixture of the restricted primitive model (RPM) of ionic fluid and neutral hard spherocylinders (HSC). To this end, we combine two theoretical…

Soft Condensed Matter · Physics 2022-07-26 M. Hvozd , T. Patsahan , O. Patsahan , M. Holovko

The scaled particle theory (SPT) approximation is applied for the study of the influence of a porous medium on the isotropic-nematic transition in a hard spherocylinder fluid. Two new approaches are developed in order to improve the…

Soft Condensed Matter · Physics 2018-04-02 M. F. Holovko , V. I. Shmotolokha

We present mode-coupling theory (MCT) results for densely packed hard-sphere fluids confined between two parallel walls and compare them quantitatively to computer simulations. The numerical solution of MCT is calculated for the first time…

Soft Condensed Matter · Physics 2023-05-10 Gerhard Jung , Thomas Franosch

We present diffusion Monte Carlo (DMC) and path-integral Monte Carlo (PIMC) calculations of a one-dimensional Bose system with realistic interparticle interactions in a periodic external potential. Our main aim is to test the predictions of…

Quantum Gases · Physics 2020-02-19 K. Dzelalija , L. Vranjes Markic

Two first-principles simulation techniques, path integral Monte Carlo (PIMC) and density functional molecular dynamics (DFT-MD), are applied to study hot, dense helium in the density-temperature range of 0.387 - 5.35 g/cc and 500 K -…

Materials Science · Physics 2015-05-13 B. Militzer

We study the lower critical solution temperature (LCST) in thermoresponsive polymer solutions by means of a coarse grained single polymer chain simulation and a theoretical approach. The simulation model includes solvent explicitly and thus…

Soft Condensed Matter · Physics 2016-11-30 G. Swaminath Bharadwaj , P. B. Sunil Kumar , Shigeyuki Komura , Abhijit P. Deshpande

The thermodynamic stability of the hard-sphere gas has been examined, using the formalism of scaled particle theory [SPT], and by applying explicitly the conditions of stability required by both the second and third laws of thermodynamics.…

Statistical Mechanics · Physics 2007-05-23 J. F. Kenney

We have obtained by Monte Carlo NVT simulations the constant-volume excess heat capacity of square-well fluids for several temperatures, densities and potential widths. Heat capacity is a thermodynamic property much more sensitive to the…

Statistical Mechanics · Physics 2007-05-23 J. Largo , J. R. Solana , L. Acedo , A. Santos

We apply the Barker-Henderson (BH) perturbation theory to the study of a Lennard-Jones fluid confined in a random porous matrix formed by hard sphere particles. In order to describe the reference system needed in this perturbation scheme,…

Soft Condensed Matter · Physics 2015-04-07 M. F. Holovko , T. M. Patsahan , V. I. Shmotolokha

We study the structural and thermodynamic properties of a model of point particles interacting by means of a Gaussian pair potential first introduced by Stillinger [Stillinger F H 1976 J. Chem. Phys. 65, 3968]. By employing integral…

Soft Condensed Matter · Physics 2009-10-31 A. Lang , C. N. Likos , M. Watzlawek , H. Lowen

We study the glassy transition for simple liquids in the hypernetted chain (HNC) approximation by means of an effective potential recently introduced. Integrating the HNC equations for hard spheres, we find a transition scenario analogous…

Statistical Mechanics · Physics 2009-10-30 Miguel Cardenas , Silvio Franz , Giorgio Parisi