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We use molecular simulations of an ionic liquid in contact with a range of nanoporous carbons to investigate correlations between ion size, pore size, pore topology and properties of the adsorbed ions. We show that diffusion coefficients…

Materials Science · Physics 2020-02-21 El Hassane Lahrar , Anouar Belhboub , Patrice Simon , Céline Merlet

Surface sensitive synchrotron x-ray scattering studies were performed to obtain the distribution of monovalent ions next to a highly charged interface. A lipid phosphate (dihexadecyl hydrogen-phosphate) was spread as a monolayer at the…

Soft Condensed Matter · Physics 2007-05-23 Wei Bu , David Vaknin , Alex Travesset

Radiative transfer coupled with highly realistic simulations of the solar atmosphere is routinely used to infer the physical properties underlying solar observations. Due to its computational efficiency, the method of short-characteristics…

Solar and Stellar Astrophysics · Physics 2018-04-17 Courtney L. Peck , Serena Criscuoli , Mark P. Rast

The diffusion of elements is a key process in understanding the unusual surface composition of white dwarfs stars and their spectral evolution. The diffusion coefficients of Paquette et al. (1986) have been widely used to model diffusion in…

Solar and Stellar Astrophysics · Physics 2020-06-17 R. A. Heinonen , D. Saumon , J. Daligault , C. E. Starrett , S. D. Baalrud , G. Fontaine

We construct a mean-field formulation of the thermodynamics of ion solvation in immiscible polar binary mixtures. Assuming an equilibrium planar interface separating two semi-infinite regions of different constant dielectric medium, we…

Soft Condensed Matter · Physics 2007-10-03 William Kung , Francisco J. Solis , Monica Olvera de la Cruz

Abstract. The present work considers a change in the momentum under the transfer of a solution through the interface. It is shown that pressure related to the partial volumes of components arises in a solution under diffusion. As a result,…

Statistical Mechanics · Physics 2021-02-16 Alex Guskov

Nonequilibrium interfacial thermodynamics is formulated in the presence of surface reactions for the study of diffusiophoresis in isothermal systems. As a consequence of microreversibility and Onsager-Casimir reciprocal relations,…

Chemical Physics · Physics 2018-12-24 Pierre Gaspard , Raymond Kapral

Solid-state ionic conduction is a key enabler of electrochemical energy storage and conversion. The mechanistic connections between material processing, defect chemistry, transport dynamics, and practical performance are of considerable…

Materials Science · Physics 2022-08-04 Andrey D. Poletayev , James A. Dawson , M. Saiful Islam , Aaron M. Lindenberg

Surface sensitive synchrotron-X-ray scattering studies reveal the distributions of monovalent ions next to highly charged interfaces. A lipid phosphate (dihexadecyl hydrogen-phosphate) was spread as a monolayer at the air-water interface,…

Soft Condensed Matter · Physics 2009-11-11 Wei Bu , David Vaknin , Alex Travesset

Turing patterns are stationary, wave-like structures that emerge from the nonequilibrium assembly of reactive and diffusive components. While they are foundational in biophysics, their classical formulation relies on a single characteristic…

Soft Condensed Matter · Physics 2026-01-30 Siamak Mirfendereski , Ankur Gupta

We analyze point defect bulk and surface diffusion near the crystal-vacuum interface and show that bulk diffusion is altered by atomic reactions at the surface-vacuum boundary. A new atomic mechanism for point defect generation and…

Materials Science · Physics 2024-06-12 Sergey Kosolobov

A thin oxide layer protects metals from electrochemical corrosion and hence the stability of this oxide layer is crucial for corrosion resistance of metals. The dynamics of cationic and anionic point defects which are injected into this…

Materials Science · Physics 2019-01-01 K. Ragavendran , Bosco Emmanuel

Ion bombardment is known to enhance surface diffusion and affect the surface morphology. To quantify this phenomenon we calculate the ion-induced diffusion constant and its dependence on the ion energy, flux and angle of incidence. We find…

Materials Science · Physics 2009-10-30 Maxim A. Makeev , Albert-Laszlo Barabasi

The diffusive transport of biased Brownian particles in a two-dimensional symmetric channel is investigated numerically considering both the no-flow and the reflection boundary conditions at the channel boundaries. Here, the geometrical…

Soft Condensed Matter · Physics 2019-09-10 Narender Khatri , P. S. Burada

The consistent description of kinetic and hydrodynamic processes is applied to the study of ion transport processes in the ionic solution-porous medium system. A system of equations is obtained for the nonequilibrium single-ion distribution…

Statistical Mechanics · Physics 2025-06-26 P. P. Kostrobij , B. M. Markovych , O. V. Viznovych , M. V. Tokarchuk

We study ion condensation onto a patterned surface of alternating charges. The competition between self-energy and ion-surface interactions leads to the formation of ionic crystalline structures at low temperatures. We consider different…

Statistical Mechanics · Physics 2009-11-13 Yuri S. Velichko , Francisco J. Solis , Sharon M. Loverde , Monica Olvera de la Cruz

A modified Poisson-Nernst-Planck system in a bounded domain with mixed Dirichlet-Neumann boundary conditions is analyzed. It describes the concentrations of ions immersed in a polar solvent and the correlated electric potential due to the…

Analysis of PDEs · Mathematics 2023-05-25 Ansgar Jüngel , Annamaria Massimini

Describing particle transport at the macroscopic or mesoscopic level in non-ideal environments poses fundamental theoretical challenges in domains ranging from inter and intra-cellular transport in biology to diffusion in porous media. Yet,…

Statistical Mechanics · Physics 2013-09-11 Marta Galanti , Duccio Fanelli , Francesco Piazza

When an ionic liquid adsorbs onto a porous electrode, its ionic arrangement is deeply modified due to a screening of the Coulombic interactions by the metallic surface and by the confinement imposed upon it by the electrode's morphology. In…

The linear response description for impurity diffusion in a granular fluid undergoing homogeneous cooling is developed in the preceeding paper. The formally exact Einstein and Green-Kubo expressions for the self-diffusion coefficient are…

Soft Condensed Matter · Physics 2009-11-07 James Lutsko , J. Javier Brey , James W. Dufty