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Related papers: Photothermal Absorption Spectroscopy of Individual…

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Current methods for producing single-walled carbon nanotubes (SWNTs) lead to heterogeneous samples containing mixtures of metallic and semiconducting species with a variety of lengths and defects. Optical detection at the single nanotube…

We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual nonfluorescent nanoclusters and nanocrystals. A 2 order of magnitude improvement of the signal is achieved compared to previous methods. This…

Optics · Physics 2007-05-23 Stéphane Berciaud , Laurent Cognet , Gerhard A Blab , Brahim Lounis

We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual non-fluorescent nano-objects. A two orders of magnitude improvement of the signal is achieved compared to previous methods. This allows for…

Other Condensed Matter · Physics 2007-05-23 Stephane Berciaud , Laurent Cognet , Gerhard Blab , Brahim Lounis

The photothermal heterodyne imaging technique enabled studies of individual weakly absorbing nano-objects in various environments. It uses a photo-induced change in the refractive index of the environment. Taking advantage of the dramatic…

Absorption microscopy is a powerful technique, enabling the detection of single non- fluorescent molecules at room temperature. So far, the molecular absorption has been probed optically via the attenuation of a probing laser. The…

Applied Physics · Physics 2018-11-21 Miao-Hsuan Chien , Mario Brameshuber , Gerhard J. Schütz , Silvan Schmid

We present the theoretical and detailed experimental characterizations of Photothermal Heterodyne Imaging. An analytical expression of the photothermal heterodyne signal is derived using the theory of light scattering from a fluctuating…

In nanomechanical photothermal absorption spectroscopy and microscopy, the measured substance becomes a part of the detection system itself, inducing a nanomechanical resonance frequency shift upon thermal relaxation. Suspended,…

Instrumentation and Detectors · Physics 2023-06-30 Robert G. West , Kostas Kanellopulos , Silvan Schmid

We consider the free carrier dispersion effect in a semiconductor nanocavity in the limit of discrete photoexcited electron-hole pairs. This analysis reveals the possibility of ultrafast, incoherent transduction and gain from a single…

The literature on the theory of the photothermal imaging of single nano objects is reviewed. Several models have been devised to describe the signals magnitude, phase and shape in dependence on the experimental and sample parameters…

Optics · Physics 2015-10-30 Markus Selmke , Frank Cichos

Photothermal microscopy has recently complemented single molecule fluorescence microscopy by the detection of individual nano-objects in absorption. Photothermal techniques gain their superior sensitivity by exploiting a heat induced…

Optics · Physics 2015-05-28 Markus Selmke , Marco Braun , Frank Cichos

Photothermal spectroscopy and microscopy provides a route to measure the spectral and spatial properties of individual nanoscopic absorbers, independent from scattering, extinction, and emission. The approach relies upon use of two light…

Optics · Physics 2021-04-12 Harrison J. Goldwyn , Stephan Link , David J. Masiello

We perform photoluminescence excitation measurements on individual CdSe/ZnS nanocrystal quantum dots (NCQDs) at room temperature to study optical transition energies and broadening. The observed features in the spectra are identified and…

Mesoscale and Nanoscale Physics · Physics 2014-10-17 M. Wolf , J. Berezovsky

Photon number resolving detectors play a central role in quantum optics. A key challenge in resolving the number of absorbed photons in the microwave frequency range is finding a suitable material that provides not only an appropriate band…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 Eric Chatterjee , Wei Pan , Daniel Soh

Room temperature detection of single quantum emitters has had a broad impact in fields ranging from biophysics to material science, photophysics, or even quantum optics. These experiments have exclusively relied on the efficient detection…

Other Condensed Matter · Physics 2008-02-11 P. Kukura , M. Celebrano , A. Renn , V. Sandoghdar

Transmission, reflection and absorption of electromagnetic radiation and photon dispersion law for 2D photonic crystals with superconducting elements are studied. The calculation of optical properties of photonic crystals is studied by…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. N. Poddubny , E. L. Ivchenko , Yu. E. Lozovik

Semiconductor nanowire field-effect transistors represent a promising platform for the development of room-temperature (RT) terahertz (THz) frequency light detectors due to the strong nonlinearity of their transfer characteristics and their…

We have used a photothermal technique, in which chopped light heats the front surface of a small ( ~ 1 mm2) sample and the chopping frequency dependence of thermal radiation from the back surface is measured with a liquid nitrogen cooled…

Materials Science · Physics 2016-01-20 J. W. Brill , Maryam Shahi , Marcia M. Payne , Jesper Edberg , Y. Yao , Xavier Crispin , J. E. Anthony

Photoabsorption cross sections of small sodium cluster cations (Na$_n^+$, n=3,5,7 and 9) were calculated at various temperatures with the time-dependent local-density-approximation (TDLDA) in conjunction with ab initio molecular dynamics…

Atomic and Molecular Clusters · Physics 2016-09-08 M. Moseler , H. Hakkinen , Uzi Landman

The present paper deals with the results of a research work on the optical properties of colloidal InP/ZnS nanocrystals stabilized with a heterobifunctional polyvinylpyrrolidone polymer. We have analyzed the absorption and photoluminescence…

Materials Science · Physics 2023-01-31 S. S. Savchenko , A. S. Vokhmintsev , M. S. Karabanalov , A. M. A. Henaish , I. A. Weinstein

Spectroscopic methods are a sensitive way to determine the chemical composition of potentially hazardous materials. Here, we demonstrate that thermally-tuned high-Q photonic crystal cavities can be used as a compact high-resolution on-chip…

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