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The electronic structure of the (LiYb)$^+$ molecular ion is investigated with two variants of the coupled cluster method restricted to single, double, and noniterative or linear triple excitations. Potential energy curves for the ground and…

Atomic Physics · Physics 2015-04-21 Michał Tomza , Christiane P. Koch , Robert Moszynski

We determine trapping conditions for ultracold polar molecules, where pairs of internal states experience identical trapping potentials. Such conditions could ensure that detrimental effects of inevitable inhomogeneities across an ultracold…

Atomic Physics · Physics 2015-06-12 Alexander Petrov , Constantinos Makrides , Svetlana Kotochigova

The challenge of building a scalable quantum processor requires consolidation of the conflicting requirements of achieving coherent control and preservation of quantum coherence in a large scale quantum system. Moreover, the system should…

Quantum Physics · Physics 2007-05-23 A. Andre , D. DeMille , J. M. Doyle , M. D. Lukin , S. E. Maxwell , P. Rabl , R. Schoelkopf , P. Zoller

We show that ultracold polar diatomic or linear molecules, oriented in an external electric field and mutually coupled by dipole-dipole interactions, can be used to realize the exact Heisenberg XYZ, XXZ and XY models without invoking any…

Quantum Physics · Physics 2022-11-09 Wenjing Yue , Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…

Quantum Physics · Physics 2007-05-23 Christiane P. Koch , José P. Palao , Ronnie Kosloff , Françoise Masnou-Seeuws

The transfer of weakly bound KRb molecules from levels just below the dissociation threshold into the vibrational ground state with shaped laser pulses is studied. Optimal control theory is employed to calculate the pulses. The complexity…

Atomic Physics · Physics 2011-04-15 Mamadou Ndong , Christiane P. Koch

We propose a new type of Feshbach resonance occurring when two different ultracold atoms in their ground state undergo an s-wave collision in the presence of a continuous-wave laser light. The atoms collide in the dissociation continuum of…

Ultracold gases in optical lattices are of great interest, because these systems bear a great potential for applications in quantum simulations and quantum information processing, in particular when using particles with a long-range…

Statistical Mechanics · Physics 2007-05-23 T. Volz , N. Syassen , D. M. Bauer , E. Hansis , S. Dürr , G. Rempe

We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a…

We report the production of $^{87}$RbCs Feshbach molecules in a crossed-beam dipole trap. A mixture of $^{87}$Rb and $^{133}$Cs is cooled close to quantum degeneracy before an interspecies Feshbach resonance at 197\,G is used to associate…

This review describes recent experimental and theoretical advances in forming molecules in ultracold gases of trapped alkali metal atoms, both by magnetic tuning through Feshbach resonances and by photoassociation. Molecular Bose-Einstein…

Chemical Physics · Physics 2007-05-23 Jeremy M. Hutson , Pavel Soldan

Ultracold polar molecules offer strong electric dipole moments and rich internal structure, which makes them ideal building blocks to explore exotic quantum matter, implement novel quantum information schemes, or test fundamental symmetries…

The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…

Atomic Physics · Physics 2015-05-27 Seth T. Rittenhouse , M. Mayle , P. Schmelcher , H. R. Sadeghpour

We theoretically study collisions between ultracold polar molecules that are polarized by microwave or static electric fields. We systematically study the dependence on field strength, microwave polarization, and detuning from rotational…

Atomic Physics · Physics 2022-02-09 Tijs Karman , Zoe Z. Yan , Martin Zwierlein

Polarized atomic ensembles play a crucial role in precision measurements. We demonstrate a novel method of creating atomic polarization in an alkali vapor in a continuous-wave regime. The method relies on a combination of optical pumping by…

Atomic Physics · Physics 2021-10-22 A. Tretiakov , C. A. Potts , Y. Y. Lu , J. P. Davis , L. J. LeBlanc

Doubly polar molecules, possessing an electric dipole moment and a magnetic dipole moment, can strongly couple to both an external electric field and a magnetic field, providing unique opportunities to exert full control of the system…

Atomic Physics · Physics 2019-11-06 Hui Li , Goulven Quéméner , Jean-François Wyart , Olivier Dulieu , Maxence Lepers

We report on the creation of ultracold heteronuclear molecules assembled from fermionic 40K and bosonic 87Rb atoms in a 3D optical lattice. Molecules are produced at a heteronuclear Feshbach resonance both on the attractive and the…

Statistical Mechanics · Physics 2007-05-23 C. Ospelkaus , S. Ospelkaus , L. Humbert , P. Ernst , K. Sengstock , K. Bongs

We propose a new method for the production of ultracold molecular ions. This method utilizes sympathetic cooling due to the strong collisions between appropriately chosen molecular ions and laser-cooled neutral atoms to realize ultracold,…

Atomic Physics · Physics 2009-11-13 Eric R. Hudson

We present a method for the creation and control of cold molecules that involves coherently combining Feshbach Resonances and STIRAP. We present analytical and numerical results showing how to optimize this process that can be implemented…

Atomic Physics · Physics 2019-10-09 Phillip Price , Susanne Yelin

We have investigated magnetically tunable Feshbach resonances in ultracold collisions of Rb with Yb in its metastable $^3$P$_2$ and $^3$P$_0$ states, using coupled-channel scattering and bound-state calculations. For the $^3$P$_2$ state, we…

Atomic Physics · Physics 2022-02-11 Bijit Mukherjee , Matthew D. Frye , Jeremy M. Hutson
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