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Electron energy loss spectroscopy (EELS) can be used to probe plasmon excitations in nanostructured materials with atomic-scale spatial resolution. For structures smaller than a few nanometers quantum effects are expected to be important,…

Mesoscale and Nanoscale Physics · Physics 2013-01-03 Kirsten Andersen , Karsten W. Jacobsen , Kristian S. Thygesen

Fluids confined in nanopores are ubiquitous in nature and technology. In recent years, the interest in confined fluids has grown, driven by research on unconventional hydrocarbon resources -- shale gas and shale oil, much of which are…

Soft Condensed Matter · Physics 2021-11-16 C. D. Dobrzanski , B. Gurevich , G. Y. Gor

A method for the evaluation of the angular width of an electron beam generated by a nanoconstriction is proposed and demonstrated. The approach is based on analysis of a narrow-width electron flow, that quantizes into modes inside a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 R. N. Gurzhi , A. N. Kalinenko , A. I. Kopeliovich , A. V. Yanovsky , E. N. Bogachek , Uzi Landman

As the continual experimental advances made in Electron energy loss spectroscopy (EELS) and cathodoluminescence (CL) open the door to practical exploitations of plasmonic effects in metal nanoparticles, there is an increasing need for…

Mesoscale and Nanoscale Physics · Physics 2016-05-31 Yu Luo , Matthias Kraft , J. B. Pendry

Strong nanoscale light-matter interaction is often accompanied by ultra-confined photonic modes and large momentum polaritons existing far beyond the light cone. A direct probe of such phenomena is difficult due to the momentum mismatch of…

On- and off-axis electron energy loss spectroscopy (EELS) is a powerful method for probing local electronic structure on single atom level. However, many materials undergo electron-beam induced transformation during the scanning…

Materials Science · Physics 2023-10-23 Kevin M. Roccapriore , Riccardo Torsi , Joshua Robinson , Sergei V. Kalinin , Maxim Ziatdinov

A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

Atomic Physics · Physics 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Understanding the stability mechanism of surface micro/nanobubbles adhered to gas-evolving electrodes is essential for improving the efficiency of water electrolysis, which is known to be hindered by the bubble coverage on electrodes. Using…

Fluid Dynamics · Physics 2024-04-16 Yixin Zhang , Xiaojue Zhu , Jeffery A. Wood , Detlef Lohse

In the quest for dynamic multimodal probing of a material's structure and functionality, it is critical to be able to quantify the chemical state on the atomic and nanoscale using element specific electronic and structurally sensitive tools…

Photonic modes in dielectric nanostructures, e.g., wide gap semiconductor like CeO2 (ceria), has potential for various applications such as light harvesting and information transmission. To fully understand the properties of such phenomenon…

Optics · Physics 2024-08-06 Yifan Wang , Shize Yang , Peter A. Crozier

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

Fundamental mechanisms of energy storage, corrosion, sensing, and multiple biological functionalities are directly coupled to electrical processes and ionic dynamics at solid-liquid interfaces. In many cases, these processes are spatially…

Materials Science · Physics 2017-01-25 Liam Collins , Jason Kilpatrick , Sergei V. Kalinin , Brian J. Rodriguez

Within Density Functional Theory, we have calculated the energy of the transitions from the ground state to the first two excited states in the electron bubbles in liquid helium at pressures from zero to about the solidification pressure.…

Soft Condensed Matter · Physics 2016-08-16 Víctor Grau , Manuel Barranco , Ricardo Mayol , Martí Pi

Doping inhomogeneities in solids are not uncommon, but their microscopic observation and understanding are limited due to the lack of bulk-sensitive experimental techniques with high-enough spatial and spectral resolution. Here, we…

The properties of helium-filled nanopores in amorphous silicon are elucidated by combining theoretical knowledge of helium electronic structure with the results of Scanning Transmission electron microscopy/electron energy loss spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2024-07-08 Bertrand Lacroix , Asunción Fernández , N. C. Pyper , Alex J. W. Thom , Colm T. Whelan

Discrete particle simulation, a combined approach of computational fluid dynamics and discrete methods such as DEM (Discrete Element Method), DSMC (Direct Simulation Monte Carlo), SPH (Smoothed Particle Hydrodynamics), PIC…

Fluid Dynamics · Physics 2014-06-20 Limin Wang , Bo Zhang , Xiaowei Wang , Wei Ge , Jinghai Li

Micro-Electro-Mechanical Systems (MEMS) normally have fixed or moving structures with cross-sections of the order of microns ($\mu m$) and lengths of the order of tens or hundreds of microns. These structures are often plates or array of…

Computational Physics · Physics 2007-05-23 N. Majumdar , S. Mukhopadhyay

We describe the thermodynamic state of a single-phase fluid confined to a porous medium with Hill's thermodynamics of small systems, also known as nanothermodynamics. This way of defining small system thermodynamics, with a separate set of…

Chemical Physics · Physics 2022-02-01 Olav Galteland , Michael T. Rauter , Kevin K. Varughese , Dick Bedeaux , Signe Kjelstrup

Conduction electrons in metallic nano-objects ($\rm 1\,nm = 10^{-9}\, m$) behave as mobile negative charges confined by a fixed positively-charged background, the atomic ions. In many respects, this electron gas displays typical plasma…

Mesoscale and Nanoscale Physics · Physics 2019-06-20 Giovanni Manfredi , Paul-Antoine Hervieux , Jérôme Hurst

Nanobubbles formed in monolayers of transition metal dichalcogenides (TMDCs) on top of a substrate feature localized potentials, in which electrons can be captured. We show that the captured electronic density can exhibit a non-trivial…

Mesoscale and Nanoscale Physics · Physics 2021-12-22 Roberto Rosati , Frank Lengers , Christian Carmesin , Matthias Florian , Tilmann Kuhn , Frank Jahnke , Michael Lorke , Doris E. Reiter