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Surface morphology of the substrate and bottom layers plays a critical role in the epitaxial growth of oxide thin films. Here, we report on the self-organized formation of a step-terrace structure in SrRuO3 (SRO) thin films grown using…

We have synthesized epitaxial Ba2IrO4 (BIO) thin-films on SrTiO3 (001) substrates by pulsed laser deposition and studied their electronic structure by dc-transport and optical spectroscopic experiments. We have observed that BIO thin-films…

Strongly Correlated Electrons · Physics 2014-04-08 J. Nichols , O. B. Korneta , J. Terzic , G. Cao , J. W. Brill , S. S. A. Seo

Barium titanate (BaTiO$_3$) is a compelling material for integrated photonics due to its strong electro-optic and second-order nonlinear properties. Crystal Ion Slicing (CIS) presents a scalable and CMOS-compatible route for fabricating…

Control over crystallographic orientation in metal-organic framework (MOF) thin films is crucial for exploiting their anisotropic properties in sensing, catalysis, and separation. Achieving reproducible, highly oriented films remains…

Recent works have shown that the domain walls of room-temperature multiferroic BiFeO3 (BFO) thin films can display distinct and promising functionalities. It is thus important to understand the mechanisms underlying domain formation in…

Materials Science · Physics 2015-05-14 C. J. M. Daumont , S. Farokhipoor , A. Ferri , J. C. Wojdel , Jorge Iniguez , B. J. Kooi , B. Noheda

Ultrathin topological insulator membranes are building blocks of exotic quantum matter. However, traditional epitaxy of these materials does not facilitate stacking in arbitrary orders, while mechanical exfoliation from bulk crystals is…

Multiferroic BiFeO3 (BFO) / La0.7Sr0.3MnO3 heterostructured thin films were grown by pulsed laser deposition on polished spark plasma sintered LaAlO3 (LAO) polycrystalline substrates. Both polycrystalline LAO substrates and BFO films were…

Materials Science · Physics 2014-03-03 D. Pravarthana , M. Trassin , Jiun Haw Chu , M. Lacotte , A. David , R. Ramesh , P. A. Salvador , W. Prellier

Materials informatics exploiting machine learning techniques, e.g., Bayesian optimization (BO), has the potential to offer high-throughput optimization of thin-film growth conditions through incremental updates of machine learning models in…

We have performed x-ray photoemission spectroscopy (XPS) on thin films of (001) and (200) oriented La(0.67)Ca(0.33)MnO(3) grown on (100) and (110) SrTiO(3) substrates by off-axis sputtering. The films were examined by XPS without exposing…

Strongly Correlated Electrons · Physics 2009-10-30 P. R. Broussard , S. B. Qadri , V. C. Cestone

Surface and ferroelectric properties of PbTiO$_3$ thin films are investigated using an interatomic potential approach with parameters computed from first-principles calculations. We show that a model developed for the bulk describes…

Materials Science · Physics 2009-11-11 M. Sepliarsky , M. G. Stachiotti , R. L. Migoni

BiFeO3 thin films have been deposited on Pt/sapphire and Pt/Ti/SiO2/Si substrates with pulsed laser deposition using the same growth conditions, respectively. Au was sputtered as the top electrode. The microscopic structure of the thin film…

The crystallographic orientation of SrIrO3 surfaces is decisive for the occurrence of topological surface states. We show from DFT computations that (001) and (110) free surfaces have comparable energies, and, correspondingly, we…

Materials Science · Physics 2020-05-15 L. Fruchter , V. Brouet , F. Brisset , H. Moutaabbid , Y. Klein

The functional properties of devices based on perovskite oxides depend strongly on the growth modes that dramatically affect surface morphology and microstructure of the hetero-structured thin films. To achieve atomically flat surface…

Materials Science · Physics 2017-10-10 Bora Kim , Sang A Lee , Daehee Seol , Woo Seok Choi , Yunseok Kim

We report on the growth of epitaxial ZnO thin films and ZnO based heterostructures on sapphire substrates by laser molecular beam epitaxy (MBE). We first discuss some recent developments in laser-MBE such as flexible ultra-violet laser beam…

Materials Science · Physics 2014-01-14 Matthias Opel , Stephan Geprägs , Matthias Althammer , Thomas Brenninger , Rudolf Gross

Understanding and manipulating properties emerging at a surface or an interface require a thorough knowledge of structure-property relationships. We report a study of a prototype oxide system, La2/3Sr1/3MnO3 grown on SrTiO3(001), by…

Strongly Correlated Electrons · Physics 2019-04-11 Lina Chen , Zhen Wang , Gaomin Wang , Hangwen Guo , Mohammad Saghayezhian , Zhaoliang Liao , Yimei Zhu , E. W. Plummer , Jiandi Zhang

Surface sensitive x-ray scattering techniques with atomic scale resolution are employed to investigate the microscopic structure of the surface of three classes of liquid binary alloys: (i) Surface segregation in partly miscible binary…

Disordered Systems and Neural Networks · Physics 2007-05-23 Holger Tostmann , Elaine DiMasi , Oleg G. Shpyrko , Ben M. Ocko , Peter S. Pershan , Moshe Deutsch

Two-dimensional materials with layered structures, appropriate bandgap, and high carrier mobilities have gathered tremendous interests due to their potential applications in optoelectronic and photovoltaic devices. Here, we report the…

Materials Science · Physics 2021-09-01 Dan Mu , Wei Zhou , Yundan Liu , Jin Li , Ming Yang , Jincheng Zhuang , Yi Du , Jianxin Zhong

As-grown superconducting MgB_2 thin films have been grown on SrTiO_3(001), MgO(001), and Al_2O_3(0001) substrates by a molecular beam epitaxy (MBE) method with novel co-evaporation conditions of low deposition rate in ultra-high vacuum. The…

Superconductivity · Physics 2009-11-10 Y. Harada , M. Udsuka , Y. Nakanishi , M. Yoshizawa

We grew 20-100 nm thick films of B20 FeGe by molecular beam epitaxy and investigated the surface structures via scanning tunneling microscopy. We observed the atomic resolution of each of the four possible chemical layers in FeGe(-1-1-1).…

Mesoscale and Nanoscale Physics · Physics 2018-07-03 J. P. Corbett , T. Zhu , A. S. Ahmed , S. J. Tjung , J. J. Repicky , T. Takeuchi , R. K. Kawakami , J. A. Gupta

Crystalline symmetries have played a central role in the identification of topological materials. The use of symmetry indicators and band representations have enabled a classification scheme for crystalline topological materials, leading to…