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Two-dimensional (2D) van der Waals ferroelectrics are recognized for enabling many applications, from memory and logic to neuromorphic computing, as well as transforming other materials to control electronic phase transitions and…

The correlated-band theory implemented as a combination of the local-density approximation with the dynamical mean-field theory is applied to PuO2. An insulating electronic structure, consistent with the experimental valence-band…

Strongly Correlated Electrons · Physics 2015-03-24 Jindrich Kolorenc , Agnieszka L. Kozub , Alexander B. Shick

We address the role of electronic correlations in different kinds of band insulators by using the two-orbital Hubbard model within the dynamical mean-field theory (DMFT). An intriguing finding is that electronic correlations turn a metal…

Strongly Correlated Electrons · Physics 2025-09-11 Nagamalleswararao Dasari , Sujan K. K. , Juana Moreno , N. S. Vidhyadhiraja

We study the coherent inelastic diffraction of very weakly bound two body clusters from a material transmission grating. We show that internal transitions of the clusters can lead to new separate peaks in the diffraction pattern whose…

Quantum Physics · Physics 2009-11-07 Martin Stoll , Thorsten Koehler

We have investigated the charge dynamics of VO2 by optical reflectivity measurements. Optical conductivity clearly shows a metal-insulator transition. In the metallic phase, a broad Drude-like structure is observed. On the other hand, in…

Strongly Correlated Electrons · Physics 2009-11-11 K. Okazaki , S. Sugai , Y. Muraoka , Z. Hiroi

Based on the conventional energy band theory, an approach is presented to describe the electronic structure of crystalline insulators in the presence of a finite homogeneous electric field. The expression of polarization is derived which…

Materials Science · Physics 2009-11-10 Zhi-Rong Liu , Jian Wu , Wenhui Duan

We follow the evolution of dressed coupled mini-bands as a function of an AC field intensity, non perturbatively, for a wide field frequency range. High and low frequency limits are characterized by two different dynamic localization…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 P. H. Rivera , P. A. Schulz

Using {\it ab initio} density functional theory and single-orbital Hubbard model calculations via the density matrix renormalization group method, we systematically studied the monolayer VOI$_2$ with a $3d^1$ electronic configuration. Our…

Strongly Correlated Electrons · Physics 2021-03-31 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Gonzalo Alvarez , Elbio Dagotto

Using first-principles calculations, we study the dependence of the electronic and vibrational properties of multi-layered PbI 2 crystals on the number of layers and focus on the electronic-band structure and the Raman spectrum.…

Mesoscale and Nanoscale Physics · Physics 2018-09-26 Mehmet Yagmurcukardes , Francois M. Peeters , Hasan Sahin

The nature of insulating state driven by electronic correlations in the quarter-filled ladder compound $\alpha'$NaV$_{2}$O$_{5}$ is investigated within a cluster dynamical mean-field approach. An extended Hubbard model with first-principle…

Strongly Correlated Electrons · Physics 2009-11-07 V. V. Mazurenko , A. I. Lichtenstein , M. I. Katsnelson , I. Dasgupta , T. Saha-Dasgupta , V. I. Anisimov

The quantum phase transition between a repulsive Luttinger liquid and an insulating Peierls state is studied in the framework of the one-dimensional spinless Holstein model. We focus on the adiabatic regime but include the full quantum…

Strongly Correlated Electrons · Physics 2011-03-08 Martin Hohenadler , Holger Fehske , Fakher F. Assaad

Excitonic insulating system is studied from the viewpoints of the orbital physics in strongly correlated electron systems. An effective model Hamiltonian for low-energy electronic states is derived from the two-orbital Hubbard model with a…

Strongly Correlated Electrons · Physics 2016-05-24 Joji Nasu , Tsutomu Watanabe , Makoto Naka , Sumio Ishihara

We present a combined density-functional theory and dynamical mean-field theory (DFT+DMFT) study of the full structural phase space of rutile-based vanadium dioxide (VO$_2$), including also the less studied M2 and T phases, using an…

Strongly Correlated Electrons · Physics 2026-03-30 Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

An interacting lattice model describing the subspace spanned by a set of strongly-correlated bands is rigorously coupled to density functional theory to enable ab initio calculations of geometric and topological material properties. The…

Strongly Correlated Electrons · Physics 2019-03-26 Ryan Requist , E. K. U. Gross

The metal-insulator transition (MIT) in vanadium dioxide VO$_2$ due to V-V dimerization has been extensively discussed for decades. While it is widely acknowledged that electron correlations, Peierls instabilities, and molecular orbital…

Strongly Correlated Electrons · Physics 2024-03-12 Shunsuke Kitou , Akitoshi Nakano , Masato Imaizumi , Yuiga Nakamura , Ichiro Terasaki , Taka-hisa Arima

We present cluster-DMFT (CTQMC) calculations based on a downfolded tight-binding model in order to study the electronic structure of vanadium dioxide (VO_2) both in the low-temperature (M_1) and high-temperature (rutile) phases. Motivated…

Strongly Correlated Electrons · Physics 2015-05-18 Bence Lazarovits , Kyoo Kim , Kristjan Haule , Gabriel Kotliar

A central tenet in the theory of quantum phase transitions (QPTs) is that a nonanalyticity in the ground-state energy in the thermodynamic limit implies a QPT. Here we report on a finding that challenges this assertion. As a case study we…

Statistical Mechanics · Physics 2020-08-20 Mariana Malard , David Brandao , Paulo Eduardo de Brito , Henrik Johannesson

Appropriate consideration of the electron correlation is essential to reproduce the intriguing metal-insulator transition accompanying the Peierls-type structural transition in VO$_2$. In the density functional theory-based approach, this…

Strongly Correlated Electrons · Physics 2021-03-16 Sooran Kim

The electronic structure of the quasi-lowdimensional vanadium sulfide \bavs3 is investigated for the different phases above the magnetic ordering temperature. By means of density functional theory and its combination with dynamical-mean…

Strongly Correlated Electrons · Physics 2009-11-13 Frank Lechermann , Silke Biermann , Antoine Georges

We study the one-dimensional Holstein model with spin-1/2 electrons at half-filling. Ground state properties are calculated for long chains with great accuracy using the density matrix renormalization group method and extrapolated to the…

Condensed Matter · Physics 2009-10-31 Eric Jeckelmann , Chunli Zhang , Steven R. White