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A new quantitative theory for polyelectrolytes in salt free dilute solutions is developed. Depending on the electrostatic interaction strength, polyelectrolytes in solutions can undergo strong stretching (with polyelectrolyte dimension…

Soft Condensed Matter · Physics 2009-10-31 N. V. Brilliantov , D. V. Kuznetsov , R. Klein

We show that the interaction of an oil-dispersed colloidal particle with an oil-water interface is highly tunable from attractive to repulsive, either by varying the sign of the colloidal charge via charge regulation, or by varying the…

Soft Condensed Matter · Physics 2016-08-25 Jeffrey Everts , Sela Samin , René van Roij

Recent progress in the understanding of the effect of electrostatics in soft matter is presented. A vast amount of materials contains ions ranging from the molecular scale (e.g., electrolyte) to the meso/macroscopic one (e.g., charged…

Soft Condensed Matter · Physics 2008-12-01 Rene Messina

We study Coulomb drag between an active layer with a clean electron liquid and a passive layer with a pinned electron lattice in the regime of fast intralayer equilibration. Such a two-fluid system offers an experimentally realizable way to…

Strongly Correlated Electrons · Physics 2019-12-17 Tobias Holder

Within the Poisson-Boltzmann (PB) approach electrolytes in contact with planar, spherical, and cylindrical electrodes are analyzed systematically. The dependences of their capacitance $C$ on the surface charge density $\sigma$ and the ionic…

Soft Condensed Matter · Physics 2017-04-24 Andreas Reindl , Markus Bier , S. Dietrich

Polyelectrolyte complexation plays an important role in materials science and biology. The internal structure of the resultant polyelectrolyte complex (PEC) phase dictates properties such as physical state, response to external stimuli, and…

In this work, we explore the statistical physics of colloidal particles that interact with electrolytes via ion-specific interactions. Firstly we study particles interact weakly with electrolyte using linear response theory. We find that…

Soft Condensed Matter · Physics 2016-10-12 Mingnan Ding , Yihao Liang , Xiangjun Xing

The advancement of fabrication and lithography techniques of semiconductors have made it possible to study bi-layer systems made of two electronic layers separated by distances of several hundred Angstroms. In this situation the electrons…

Strongly Correlated Electrons · Physics 2009-10-31 A. G. Rojo

The interaction of an electron with a local static charge distribution (e.g., an atom or molecule) is dominated at large distances by the radial 1/r Coulomb potential. The second order effect comes from the non-central electric dipole…

Quantum Physics · Physics 2023-02-08 A. D. Alhaidari , H. Bahlouli

We consider a class of systems where, due to the large mismatch of dielectric constants, the Coulomb interaction is approximately one-dimensional. Examples include ion channels in lipid membranes and water filled nanopores in silicon or…

Statistical Mechanics · Physics 2015-06-25 A. Kamenev , J. Zhang , A. I. Larkin , B. I. Shklovskii

We propose a semi-empirical formula for the cross section of ionization by electron impact. The formula involves adjustable parameters which are determined by comparison with measured or numerically calculated cross sections. In the latter…

Atomic Physics · Physics 2024-04-09 Djamel Benredjem , Jean-Christophe Pain

The activity coefficient of ions in solution was proposed by Bjerrum (1916) to depend on the cube root of concentration, because of a good fit with data for low and moderate salt concentration. However, Debye and H\"uckel (DH) later…

Chemical Physics · Physics 2024-03-05 P. M. Biesheuvel

We study the attractive interactions between rod-like charged polymers in solution that appear in the presence of multi-valence counterions. The counterions condensed to the rods exhibit both a strong transversal polarization and a…

Soft Condensed Matter · Physics 2009-10-31 Francisco J. Solis , Monica Olvera de la Cruz

This paper discusses the little-known fact that Donnan's equilibrium criteria established over 100 years ago neglected the coupling between ion concentrations and the osmotic pressure. Such coupling can be treated based on general…

Chemical Physics · Physics 2021-11-25 Gang Chen

We provide numerical evidence that hydrodynamic interactions are screened for charged polymers in salt solution on time scales below the Zimm time. At very short times, a crossover to hydrodynamic behavior is observed. Our conclusions are…

Soft Condensed Matter · Physics 2008-10-01 Jens Smiatek , Friederike Schmid

We formulate a general mean-field theory of a flat electric double layer in ionic liquids and electrolyte solutions with ions possessing static polarizability and a permanent dipole moment on a charged electrode. We establish a new…

Statistical Mechanics · Physics 2021-08-17 Yu. A. Budkov , S. V. Zavarzin , A. L. Kolesnikov

The efficiency of nanopore-based polymer sensing devices depends on the fast capture of anionic polyelectrolytes by negatively charged pores. This requires the cancellation of the electrostatic barrier associated with repulsive polymer-pore…

Soft Condensed Matter · Physics 2017-10-25 Sahin Buyukdagli , Tapio Ala-Nissila

A simple model is presented for the appearance of attraction between two like charged polyions inside a polyelectrolyte solution. The polyions are modeled as rigid cylinders in a continuum dielectric solvent. The strong electrostatic…

Soft Condensed Matter · Physics 2009-10-31 Alexandre Diehl , Humberto A. Carmona , Yan Levin

The dependence of the lower critical solution temperature (LCST) of charged, thermosensitive copolymers on their charge fraction and the salt concentration is investigated by employing systematic cloud-point experiments and analytical…

Soft Condensed Matter · Physics 2015-06-17 Jan Heyda , Sebastian Soll , Jiayin Yuan , Joachim Dzubiella

The Coulomb interaction between the two protons is included in the calculation of proton-deuteron elastic scattering, radiative proton-deuteron capture and two-body electromagnetic disintegration of ${}^3\mathrm{He}$. The hadron dynamics is…

Nuclear Theory · Physics 2009-11-11 A. Deltuva , A. C. Fonseca , P. U. Sauer
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