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Hybrid density functional theory (DFT) remains intractable for large periodic systems due to the demanding computational cost of exact exchange. We apply the tensor hypercontraction (THC) (or interpolative separable density fitting)…

Computational Physics · Physics 2023-10-13 Adam Rettig , Joonho Lee , Martin Head-Gordon

Most approximate exchange-correlation functionals used within density functional theory are constructed as the sum of two distinct contributions for exchange and correlation. Separating the exchange component from the entire functional is…

Condensed Matter · Physics 2009-10-28 Claudia Filippi , C. J. Umrigar , Xavier Gonze

As a proof of principle, self-consistent Kohn--Sham calculations are performed with the exact exchange-correlation functional. Finding the exact functional for even one trial density requires solving the interacting Schr\"odinger equation…

Chemical Physics · Physics 2014-07-14 Lucas O. Wagner , Thomas E. Baker , E. M. Stoudenmire , Kieron Burke , Steven R. White

An accurate analytical parametrization for the exchange-correlation free energy of the homogeneous electron gas, including interpolation for partial spin-polarization, is derived via thermodynamic analysis of recent restricted path integral…

Chemical Physics · Physics 2015-06-17 Valentin V. Karasiev , Travis Sjostrom , James Dufty , S. B. Trickey

Exchange interactions are a manifestation of the quantum mechanical nature of the electrons and play a key role in predicting the properties of materials from first principles. In density functional theory (DFT), a widely used approximation…

Materials Science · Physics 2020-03-27 Marco Bernardi

The engineered spin structures recently built and measured in scanning tunneling microscope experiments are calculated using density functional theory. By determining the precise local structure around the surface impurities, we find the Mn…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Chiung-Yuan Lin , B. A. Jones

A simple exact-exchange density-functional method for a quasi-two-dimensional electron gas with variable density is presented. An analytical expression for the exact-exchange potential with only one occupied subband is provided, without…

Condensed Matter · Physics 2009-11-07 F. A. Reboredo , C. R. Proetto

By generalizing the usual current density to a matrix with respect to spin variables, a general equation of continuity satisfied by the density matrix and current density matrix has been derived. This equation holds in arbitrary spin-orbit…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Hua-Tong Yang , Chengshi Liu

A recent study of Mejia-Rodriguez and Trickey [Phys. Rev. A 96, 052512 (2017)] showed that the deorbitalization procedure (replacing the exact Kohn-Sham kinetic-energy density by an approximate orbital-free expression) applied to…

Materials Science · Physics 2018-10-10 Fabien Tran , Péter Kovács , Leila Kalantari , Georg K. H. Madsen , Peter Blaha

SERF magnetometers based on dense ensembles of alkali-metal spins are precision quantum sensors that hold the record of measured and projected sensitivity to magnetic fields, in the $\mu\textrm{G}-\textrm{mG}$ range. At geomagnetic fields…

Quantum Physics · Physics 2025-05-29 Mark Dikopoltsev , Uriel Levy , Or Katz

We develop the theoretical model that describes dynamic non-equilibrium effects of external inertial and axion fields in a system of particles with spin. The possibility of using the spin density and the current density of non-relativistic…

High Energy Physics - Theory · Physics 2026-02-19 Mariya Iv. Trukhanova , Yuri N. Obukhov

We employ the combination of the density functional and the dynamical mean-field theory (LDA+DMFT) to investigate the electronic structure and magnetic properties of SrCoO3, monocrystal of which were prepared recently. Our calculations lead…

Strongly Correlated Electrons · Physics 2012-09-25 J. Kuneš , V. Křápek , N. Parragh , G. Sangiovanni , A. Toschi , A. V. Kozhevnikov

It is shown that the electron spin may not be conserved after a spin-independent scattering. This fact strongly limits the validity of the classical model of spin-up/spin-down bands, which has been used for description of magnetic…

Materials Science · Physics 2013-04-09 Vadym Zayets

The spin-orbit interaction enables interconversion between a charge current and a spin current. It is usually believed that in a nonmagnetic metal (NM) or at a NM/ferromagnetic metal (FM) bilayer interface, the symmetry of spin-orbit…

The charge and spin diffusion equations taking into account spin-flip and spin-transfer torque were numerically solved using a finite element method in complex non-collinear geometry. This approach was used to study the spin-dependent…

Mesoscale and Nanoscale Physics · Physics 2010-10-14 N. Strelkov , A. Vedyayev , D. Gusakova , L. D. Buda-Prejbeanu , M. Chshiev , S. Amara , A. Vaysset , B. Dieny

Section I presents a variety of analytical estimations related to spin coherence time (SCT) in a purely electric frozen-spin ring. The main result is that, in the case of m > 0 and vertical oscillations only, the kinetic energy equilibrium…

Accelerator Physics · Physics 2015-06-09 Yuri Orlov

While tremendous work has gone into spin-orbit torque and spin current generation, charge-to-spin conversion efficiency remains weak in silicon to date, generally stemming from the low spin-orbit coupling (low atomic number, Z) and lack of…

We present temperature-dependent atomic and magnetic pair distribution function (PDF) analysis of neutron total scattering measurements of antiferromagnetic MnO, an archetypal strongly correlated transition-metal oxide. The known…

Synthetic antiferromagnets (SAF) have been proposed to replace ferromagnets in magnetic memory devices to reduce the stray field, increase the storage density and improve the thermal stability. Here we investigate the spin-orbit torque in a…

Materials Science · Physics 2018-07-04 P. X. Zhang , L. Y. Liao , G. Y. Shi , R. Q. Zhang , H. Q. Wu , Y. Y. Wang , F. Pan , C. Song

Analytical gradients of the total energy are provided for local density and generalized-gradient hybrid approximations to generalized Kohn-Sham spin-current density functional theory (SCDFT). It is shown that gradients may be determined…

Materials Science · Physics 2023-07-21 Jacques K. Desmarais , Alessandro Erba , Jean-Pierre Flament
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