English

Will $^{37}$Ar emissions from light water power reactors become an obstacle to its use for nuclear explosion monitoring?

Instrumentation and Detectors 2020-06-05 v1 Physics and Society

Abstract

37^{37}Ar is a promising candidate for complementing radioxenon isotopes as indicators of underground nuclear explosions. This study evaluates its potential anthropogenic background caused by emissions from commercial pressurised water reactors. Various 37^{37}Ar production pathways, which result from activation of 36^{36}Ar and of 40^{40}Ca, respectively, are identified and their emissions quantified. In-core processes include (1) the restart of operation and degassing of the primary cooling water after maintenance and refueling shutdown, (2) the replacement of primary coolant water for limiting its tritium concentrations, and (3) the leakage of 37^{37}Ar produced from calcium impurities in UO2_{2} after fuel rod failures. Activation of air and of calcium in concrete within the biological shield are major out-of-core production pathways. Whereas emissions from in-core processes are transient, a rather constant 37^{37}Ar source term results from its out-of-core production. Generic atmospheric dispersion simulations indicate that already at moderate distances from the emitter, concentrations of 37^{37}Ar caused by routine reactor operations are far below its cosmogenic background in air. The only exception results from an inadvertent reactor re-start without operation of the primary cooling water degassing system for prolonged time. Such an event also causes high emissions of 41^{41}Ar which can be used for discriminating its 37^{37}Ar signal from an underground nuclear explosion.

Keywords

Cite

@article{arxiv.2006.02823,
  title  = {Will $^{37}$Ar emissions from light water power reactors become an obstacle to its use for nuclear explosion monitoring?},
  author = {Gerald Kirchner and Franziska Gerfen and Anna Heise and Timo Schlüschen},
  journal= {arXiv preprint arXiv:2006.02823},
  year   = {2020}
}

Comments

14 pages, 2 tables, 9 figures