English

Weak low-temperature ferromagnetism and linear magnetoresistance in Lu$_{0.75}$Fe$_6$Sn$_6$ with a disordered HfFe$_6$Ge$_6$-type structure

Materials Science 2025-07-16 v1 Strongly Correlated Electrons

Abstract

We report the synthesis of Lu0.75_{0.75}Fe6_6Sn6_6 single crystals with a Fe-kagome lattice using a self-flux method. The crystal structure, magnetic, thermodynamic and electrical transport properties were investigated. Structure refinement reveals that Lu0.75_{0.75}Fe6_6Sn6_6 has a HfFe6_6Ge6_6-type structure as the major framework intergrown with a CoSn-type structure, leading to a vacancy of 25% on the Lu-site and disorder on the Sn-site. It exhibits a significant magnetic anisotropy with weak ferromagnetism in the ab-plane below 40 K and antiferromagnetic behavior along the c-axis. The weak ferromagnetism is due to the canted antiferromagnetism with magnetic moment deviating from the cc-axis to the ab-plane. Besides, an anisotropic non-saturated linear magnetoresistance is also observed in Lu0.75_{0.75}Fe6_6Sn6_6, probably resulting from the structural disorder in the sample.

Keywords

Cite

@article{arxiv.2507.10964,
  title  = {Weak low-temperature ferromagnetism and linear magnetoresistance in Lu$_{0.75}$Fe$_6$Sn$_6$ with a disordered HfFe$_6$Ge$_6$-type structure},
  author = {Chenfei Shi and Zhaodi Lin and Qiyuan Liu and Junai Lv and Xiaofan Xu and Baojuan Kang and Jin-Hu Yang and Yi Liu and Jian Zhang and Shixun Cao and Jin-Ke Bao},
  journal= {arXiv preprint arXiv:2507.10964},
  year   = {2025}
}

Comments

20 pages, 6 figures