English

Unravelling the role of phoretic and hydrodynamic interactions in active colloidal suspensions

Soft Condensed Matter 2019-06-26 v2

Abstract

Active fluids comprise a variety of systems composed of elements immersed in a fluid environment which can convert some form of energy into directed motion; as such they are intrinsically out-of-equilibrium in the absence of any external forcing. A fundamental problem in the physics of active matter concerns the understanding of how the characteristics of the autonomous propulsion and agent-agent interactions determine the collective dynamics of the system. We study numerically suspensions of self-propelled diffusiophoretic colloids, in (quasi)-2d configurations, accounting for both dynamically resolved solute-mediated phoretic interactions and solvent-mediated hydrodynamic interactions. Our results show that the system displays different scenarios at changing the colloid-solute affinity and it develops a cluster phase in the chemoattractive case. We study the statistics of cluster sizes and cluster morphologies for different magnitudes of colloidal activity. Finally, we provide evidences that hydrodynamics plays a relevant role in the aggregation kinetics and cluster morphology, significantly hindering the cluster growth.

Keywords

Cite

@article{arxiv.1605.03773,
  title  = {Unravelling the role of phoretic and hydrodynamic interactions in active colloidal suspensions},
  author = {Andrea Scagliarini and Ignacio Pagonabarraga},
  journal= {arXiv preprint arXiv:1605.03773},
  year   = {2019}
}