Universal Thickness-Dependent Absorption in Solids at the Nanoscale
Abstract
Through systematic experimental and theoretical studies of layer-thickness-dependent absorption in semiconducting MoSe and WS across the visible to near-infrared spectral range, we demonstrate a universal absorption behavior in solids at nanoscale thicknesses. With increasing thickness, a non-monotonic evolution of absorption integrated over the measured spectral region is revealed which is accompanied by pronounced oscillatory features. This strongly deviates from the expected Beer-Lambert law. The observed behavior has origins in the electromagnetic interference effects taking place between the two surfaces of the thin crystals. The present work on 2D semiconductors is extendable to all kinds of solids such as conventional semiconductors (e.g. Si, GaAs, GaN, InP), (semi)metals (e.g. Al, Ag, Au, c-HOPG) and 2D magnetic materials (e.g. CrSBr and NiPS). Our results provide fundamental insights into light-matter interactions in solids at the nanoscale and are vital for optimally designing the new generation of absorption-based flexible optoelectronic devices.
Cite
@article{arxiv.2510.21354,
title = {Universal Thickness-Dependent Absorption in Solids at the Nanoscale},
author = {Bhumika Chauhan and Nikhil Singh and Subhrajit Dalai and Abhisek Saidarsan and Sayantan Patra and Sourabh Jain and Aparna Deshpande and Ashish Arora},
journal= {arXiv preprint arXiv:2510.21354},
year = {2025}
}
Comments
11 pages, 4 figures in main text, 12 figures in supplementary materials