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Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation

Strongly Correlated Electrons 2025-08-11 v1

Abstract

Bose-Einstein condensation (BEC), a macroscopic quantum phenomenon arising from phase coherence and bosonic statistics, has been realized in quantum magnets. Here, we report the observation of a universal magnetocaloric effect (MCE) near a BEC quantum critical point (QCP) in copper sulfate crystal (CuSO45H2OCuSO_4 \cdot 5H_2O). By conducting magnetocaloric and nuclear magnetic resonance measurements, we uncover a field-driven BEC QCP, evidenced by the universal scaling law Tc(BcB)2/3T_c \propto (B_c - B)^{2/3} and the perfect data collapse of the magnetic Gr\"uneisen ratio. Thermal excitation triggers a dimensional crossover to a 1D quantum-critical regime, where the MCE scaling strictly matches the universality class of 1D Fermi gases. Notably, the quantum-critical MCE enables cooling down to 12.8 mK without helium-3, with very fast thermal relaxation rate that is critical for high cooling power. This work demonstrates the universal MCE in magnon BEC systems, using a common copper sulfate compound as a paradigmatic example, and paves the way for next-generation sub-Kelvin cooling.

Keywords

Cite

@article{arxiv.2508.05750,
  title  = {Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation},
  author = {Junsen Xiang and Enze Lv and Qinxin Shen and Cheng Su and Xuetong He and Yinghao Zhu and Yuan Gao and Xin-Yang Liu and Dai-Wei Qu and Xinlei Wang and Xi Chen and Qian Zhao and Haifeng Li and Shuo Li and Jie Yang and Jun Luo and Peijie Sun and Wentao Jin and Yang Qi and Rui Zhou and Wei Li and Gang Su},
  journal= {arXiv preprint arXiv:2508.05750},
  year   = {2025}
}

Comments

20 pages, 15 figures