English

Unexpected Magnetism in Alkaline Earth Mono-Silicides

Other Condensed Matter 2012-09-18 v2

Abstract

Alkaline earth mono-silicides ({\AE}Si, {\AE} == Ca, Sr, Ba) are poor metals and their transport properties are not solely determined by the Zintl anion, in contrast to their Zintl-type composition. Their conducting network is formed by the depopulated 1{}^{1}_{\infty}[Si2^{2-}] π\pi-system and {\AE}-dd states. This justifies the special local coordination of the metal atoms and the planarity of the silicon chains. The low density of carriers seems to be a playground for magnetic instabilities and the triangular prismatic arrangement of {\AE} atoms responsible for the observed weak glassy behavior.

Keywords

Cite

@article{arxiv.0909.0434,
  title  = {Unexpected Magnetism in Alkaline Earth Mono-Silicides},
  author = {Eduardo Cuervo-Reyes and Elizabeth Diane Stalder and Christian Mensing and Serhiy Budnyk and Reinhard Nesper},
  journal= {arXiv preprint arXiv:0909.0434},
  year   = {2012}
}

Comments

preprint form: 18 pages, 8 figures, 2 tables