Hidden states of matter with novel and unusual properties may be created if a system out of equilibrium can be induced to follow a trajectory to a state which is inaccessible or does not even exist under normal equilibrium conditions. Here we report on the discovery of a hidden (H) topologically protected electronic state in a layered dichalcogenide 1T-TaS2 crystal reached as a result of a quench caused by a single 35 fs laser pulse. The properties of the H state are markedly different from any other state of the system: it exhibits a large drop of electrical resistance, strongly modified single particle and collective mode spectra and a marked change of optical reflectivity. Particularly important and unusual, the H state is stable for an arbitrarily long time until a laser pulse, electrical current or thermal erase procedure is applied, causing it to revert to the thermodynamic ground state. Major observed events can be reproduced by a kinetic model describing the conversion of photo excited electrons and holes into an electronically ordered crystal, thus converting a Mott insulator to a conducting H state. Its long-time stability follows from the topological protection of the number of periods in the electronic crystal.
@article{arxiv.1401.6786,
title = {Ultrafast switching to a stable hidden topologically protected quantum state in an electronic crystal},
author = {L. Stojchevska and I. Vaskivskyi and T. Mertelj and P. Kusar and D. Svetin and S. Brazovskii and D. Mihailovic},
journal= {arXiv preprint arXiv:1401.6786},
year = {2016}
}
Comments
21 pages and 5 figures, separate supplementary material