Low-energy coherent charge-density wave excitations are investigated in blue bronze (K0.3MoO3) and red bronze (K0.33MoO3) by femtosecond pump-probe spectroscopy. A linear gapless, acoustic-like dispersion relation is observed for the transverse phasons with a pronounced anisotropy in K0.33MoO3. The amplitude mode exhibits a weak (optic-like) dispersion relation with a frequency of 1.67 THz at 30 K. Our results show for the first time that the time-resolved optical technique provides momentum resolution of collective excitations in strongly correlated electron systems.Low-energy coherent charge-density wave excitations are investigated in blue bronze (K0.3MoO3) and red bronze (K0.33MoO3) by femtosecond pump-probe spectroscopy. A linear gapless, acoustic-like dispersion relation is observed for the transverse phasons with a pronounced anisotropy in K0.33MoO3. The amplitude mode exhibits a weak (optic-like) dispersion relation with a frequency of 1.67 THz at 30 K. Our results show for the first time that the time-resolved optical technique provides momentum resolution of collective excitations in strongly correlated electron systems.
@article{arxiv.cond-mat/0310357,
title = {Ultrafast Collective Dynamics in the Charge-Density-Wave Conductor K$_{0.3}$MoO$_{3}$},
author = {Yuhang Ren and Zhu'an Xu and Gunter L\U{fc}pke},
journal= {arXiv preprint arXiv:cond-mat/0310357},
year = {2009}
}