Tunable Spin-Orbit Torques in Cu-Ta Binary Alloy Heterostructures

The spin Hall effect (SHE) is found to be strong in heavy transition metals (HM), such as Ta and W, in their amorphous and/or high resistivity form. In this work, we show that by employing a Cu-Ta binary alloy as buffer layer in an amorphous Cu$_{100-x}$Ta$_{x}$-based magnetic heterostructure with perpendicular magnetic anisotropy (PMA), the SHE-induced damping-like spin-orbit torque (DL-SOT) efficiency $|\xi_{DL}|$ can be linearly tuned by adjusting the buffer layer resistivity. Current-induced SOT switching can also be achieved in these Cu$_{100-x}$Ta$_{x}$-based magnetic heterostructures, and we find the switching behavior better explained by a SOT-assisted domain wall propagation picture. Through systematic studies on Cu$_{100-x}$Ta$_{x}$-based samples with various compositions, we determine the lower bound of spin Hall conductivity $|\sigma_{SH}|\approx2.02\times10^{4}[\hbar/2e]\Omega^{-1}\cdot\operatorname{m}^{-1}$ in the Ta-rich regime. Based on the idea of resistivity tuning, we further demonstrate that $|\xi_{DL}|$ can be enhanced from 0.087 for pure Ta to 0.152 by employing a resistive TaN buffer layer.