English

Topological Insulator in Twisted Transition Metal Dichalcogenide Heterotrilayers

Mesoscale and Nanoscale Physics 2025-08-08 v2

Abstract

The quantum spin Hall effect has been predicted in twisted homobilayer transition metal dichalcogenides (TMDs) owing to the layer-pseudospin magnetic field. Recently, experimental observations have also confirmed such topological states of matter. However, the topological electronic properties in multilayer moir\'e superlattices remain to be further explored. In twisted TMDs heterotrilayers, the realization of moir\'e potential with various symmetries becomes feasible. Here, we demonstrate that twisted trilayer TMDs can enter a topological insulator phase under the influence of moir\'e potential with C6{C_6} symmetry. Specifically, we built two types of trilayer heterostructures, where the low-energy valence band electrons are contributed by the middle layer. In the AA-stacked moir\'e WS2_2/WSe2_2/MoS2_2 heterotrilayers where only the middle layer is twisted, the maxima of the moir\'e potential exhibits an approximate C6{C_6} symmetry. The C6C_6 symmetry effectively compensates for the spatial inversion symmetry breaking in the WSe2_2 layer, leading to a twist-angle-dependent topological phase transition. Leveraging a Green's function approach, we calculate the local state density of edge states at topological minigaps, confirming their nature as moir\'e edge states. In the helical twisted AA-stacked moir\'e MoS2_2/WSe2_2/MoS2_2 heterotrilayers, we observed a mosaic pattern of topological and trivial insulators. The emergence of topological mosaic is attributed to the maxima of the local moir\'e potential possessing C6C_6 symmetry. The results provide a new way for the experimental realization of topological phases in TMDs heterojunctions.

Keywords

Cite

@article{arxiv.2410.05197,
  title  = {Topological Insulator in Twisted Transition Metal Dichalcogenide Heterotrilayers},
  author = {Hao He and Zhao Gong and Qing-Jun Tong and Dawei Zhai and Wang Yao and Xing-Tao An},
  journal= {arXiv preprint arXiv:2410.05197},
  year   = {2025}
}

Comments

8 pages, 6 figures