Three-point susceptibilities $\chi_n(k;t)$ and $\chi_n^s(k;t)$: mode-coupling approximation
Abstract
Recently, it was argued that a three-point susceptibility equal to the density derivative of the intermediate scattering function, , enters into an expression for the divergent part of an integrated four-point dynamic density correlation function of a colloidal suspension [Berthier \textit{et al.}, J. Chem. Phys. \textbf{126}, 184503 (2007)]. We show that, within the mode-coupling theory, the equation of motion for is essentially identical as the equation of motion for the limit of the three-point susceptibility introduced by Biroli \textit{et al.} [Phys. Rev. Lett. \textbf{97}, 195701 (2006)]. We present a numerical solution of the equation of motion for . We also derive and numerically solve an equation of motion for the density derivative of the self-intermediate scattering function, . We contrast the wave vector dependence of and .
Keywords
Cite
@article{arxiv.0810.3636,
title = {Three-point susceptibilities $\chi_n(k;t)$ and $\chi_n^s(k;t)$: mode-coupling approximation},
author = {Grzegorz Szamel and Elijah Flenner},
journal= {arXiv preprint arXiv:0810.3636},
year = {2009}
}