Three-dimensional theory for interaction between atomic ensembles and free-space light

Atomic ensembles have shown to be a promising candidate for implementations of quantum information processing by many recently-discovered schemes. All these schemes are based on the interaction between optical beams and atomic ensembles. For description of these interactions, one assumed either a cavity-QED model or a one-dimensional light propagation model, which is still inadequate for a full prediction and understanding of most of the current experimental efforts which are actually taken in the three-dimensional free space. Here, we propose a perturbative theory to describe the three-dimensional effects in interaction between atomic ensembles and free-space light with a level configuration important for several applications. The calculations reveal some significant effects which are not known before from the other approaches, such as the inherent mode-mismatching noise and the optimal mode-matching conditions. The three-dimensional theory confirms the collective enhancement of the signal-to-noise ratio which is believed to be one of the main advantage of the ensemble-based quantum information processing schemes, however, it also shows that this enhancement need to be understood in a more subtle way with an appropriate mode matching method.