English

Thermodynamics of anisotropic triangular magnets with ferro- and antiferromagnetic exchange

Strongly Correlated Electrons 2015-09-01 v1

Abstract

We investigate thermodynamic properties like specific heat cVc_{V} and susceptibility χ\chi in anisotropic J1J_1-J2J_2 triangular quantum spin systems (S=1/2S=1/2). As a universal tool we apply the finite temperature Lanczos method (FTLM) based on exact diagonalization of finite clusters with periodic boundary conditions. We use clusters up to N=28N=28 sites where the thermodynamic limit behavior is already stably reproduced. As a reference we also present the full diagonalization of a small eight-site cluster. After introducing model and method we discuss our main results on cV(T)c_V(T) and χ(T)\chi(T). We show the variation of peak position and peak height of these quantities as function of control parameter J2/J1J_2/J_1. We demonstrate that maximum peak positions and heights in N\'eel phase and spiral phases are strongly asymmetric, much more than in the square lattice J1J_1-J2J_2 model. Our results also suggest a tendency to a second side maximum or shoulder formation at lower temperature for certain ranges of the control parameter. We finally explicitly determine the exchange model of the prominent triangular magnets Cs2_2CuCl4_4 and Cs2_{2}CuBr4_{4} from our FTLM results.

Keywords

Cite

@article{arxiv.1506.09104,
  title  = {Thermodynamics of anisotropic triangular magnets with ferro- and antiferromagnetic exchange},
  author = {Burkhard Schmidt and Peter Thalmeier},
  journal= {arXiv preprint arXiv:1506.09104},
  year   = {2015}
}

Comments

13 pages, 12 figures