We apply a recently developed first-principles based approach for treating generic spin-phonon couplings in materials with strong spin-orbit coupling to study α-RuCl3. Of particular focus is the potential for this material to exhibit a phonon thermal Hall effect induced by spin-phonon interactions. We find that spin-orbit coupling significantly enriches the form of these interactions, and imbues them with chirality that is conducive to generating finite phonon Berry curvatures. We show that this leads to a phonon thermal Hall effect that qualitatively reproduces the measured field dependence of κxy without requiring a field-induced spin liquid.
@article{arxiv.2407.00660,
title = {Theory of Intrinsic Phonon Thermal Hall Effect in $\alpha$-RuCl$_3$},
author = {Ramesh Dhakal and David A. S. Kaib and Kate Choi and Sananda Biswas and Roser Valenti and Stephen M. Winter},
journal= {arXiv preprint arXiv:2407.00660},
year = {2026}
}
Comments
22 pages, 9 figures including supplemental material. Rewrite to correct errors and change format