English

The magnetic structure of Ce$_3$TiBi$_5$ and its relation to current-induced magnetization

Strongly Correlated Electrons 2024-03-11 v1 Materials Science

Abstract

The control of magnetization using electric fields has been extensively studied in magnetoelectric multiferroic insulator materials. Changes in magnetization in bulk metals caused by electric currents have attracted less attention. The recently discovered metallic magnet Ce3_3TiBi5_5 has been reported to exhibit current-induced magnetization. Here we determined the magnetic structure of Ce3_3TiBi5_5 using neutron diffraction, aiming to understand the microscopic origin of this magnetoelectric phenomenon in a metal. We established that the antiferromagnetic order emerging below TN=5T_N=5 K is a cycloid order described by P63/mcm.1(0,0,g)00sssP6_3/mcm.1'(0,0,g)00sss with small moment sizes of 0.50(2) μB0.50(2)~\mu_B and propagation vector k=(0,0,0.386){\bf k}=(0,0,0.386). Surprisingly, the symmetry of this magnetic structure is inconsistent with the presence of current-induced magnetization and potential origins of this inconsistency with previous results are discussed. Additionally, our results suggest that moments order along their hard magnetic direction in Ce3_3TiBi5_5, a phenomenon which has been observed in other Kondo systems.

Keywords

Cite

@article{arxiv.2403.04896,
  title  = {The magnetic structure of Ce$_3$TiBi$_5$ and its relation to current-induced magnetization},
  author = {Nicolas Gauthier and Romain Sibille and Vladimir Pomjakushin and Øystein S. Fjellvåg and James Fraser and Mathieu Desmarais and Andrea D. Bianchi and Jeffrey A. Quilliam},
  journal= {arXiv preprint arXiv:2403.04896},
  year   = {2024}
}

Comments

6 pages, 3 figures, accepted for publication in Phys. Rev. B as a Letter