The connection between time-local and time-nonlocal perturbation expansions
Abstract
There exist two canonical approaches to describe open quantum systems by a time-evolution equation: the Nakajima-Zwanzig quantum master equation, featuring a time-nonlocal memory kernel , and the time-convolutionless equation with a time-local generator . These key quantities have recently been shown to be connected by an exact fixed-point relation [Phys. Rev. X 11, 021041 (2021)]. Here we show that this implies a recursive relation between their perturbative expansions, allowing a series for the kernel to be translated directly into a corresponding series for the more complicated generator . This leads to an elegant way of computing the generator using well-developed, standard memory-kernel techniques for strongly interacting open systems. Moreover, it allows for an unbiased comparison of time-local and time-nonlocal approaches independent of the particular technique chosen to calculate expansions of and (Nakajima-Zwanzig projections, real-time diagrams, etc.). We illustrate this for leading and next-to-leading order calculations of and for the single impurity Anderson model using both the bare expansion in the system-environment coupling and a more advanced renormalized series. We compare the different expansions obtained, quantify the legitimacy of the generated dynamics (complete positivity) and benchmark with the exact result in the non-interacting limit.
Keywords
Cite
@article{arxiv.2107.08949,
title = {The connection between time-local and time-nonlocal perturbation expansions},
author = {K. Nestmann and M. R. Wegewijs},
journal= {arXiv preprint arXiv:2107.08949},
year = {2021}
}
Comments
14 pages, 3 figures