English

The aqueous Triton X-100 - Dodecyltrimethylammonium bromide micellar mixed system. Experimental results and thermodynamic analysis

Soft Condensed Matter 2018-09-18 v1

Abstract

The micellization process of the aqueous mixed system Triton X-100 (TX100)-Dodecyltrimethylammonium Bromide (DTAB) was studied with a battery of procedures: surface tension, static and dynamic light scattering and ion-selective electrodes. Results were also analysed with two thermodynamic procedures. The system shows some changes in its behaviour with changing the mole fraction of DTAB, αDTAB\alpha_{DTAB}, in the whole surfactant mixture. For αDTAB<0.40 \alpha_{DTAB} < 0.40 micelles are predominantly TX100 with scarce solubilized DTA+ ions, and TX100 acts as a nearly ideal solvent. In the range 0.50<αDTAB<0.750.50 < \alpha_{DTAB} < 0.75 it seems that none of the components acts as a solvent, and above αDTAB>0.75\alpha_{DTAB} > 0.75 there are abrupt changes in the size and electrophoretic mobility of micelles. These phenomena have been interpreted in the light of the thermodynamic results and some TX100-ionic surfactant mixtures of literature.

Keywords

Cite

@article{arxiv.1806.09721,
  title  = {The aqueous Triton X-100 - Dodecyltrimethylammonium bromide micellar mixed system. Experimental results and thermodynamic analysis},
  author = {Patricio Serafini and Marcos Fernández-Leyes and Jhon M. Sánchez and Romina B. Pereyra and Erica P. Schulz and Gillermo A. Durand and Pablo C. Schulz and Hernán A. Ritacco},
  journal= {arXiv preprint arXiv:1806.09721},
  year   = {2018}
}