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T-Carbon: A Novel Carbon Allotrope

Materials Science 2015-05-28 v1

Abstract

A structurally stable crystalline carbon allotrope is predicted by means of the first-principles calculations. This allotrope can be derived by substituting each atom in diamond with a carbon tetrahedron, and possesses the same space group Fd^1 3m as diamond, which is thus coined as T- carbon. The calculations on geometrical, vibrational and electronic properties reveal that T-carbon, with a considerable structural stability and a much lower density 1.50 g/cm3, is a semiconductor with a direct band gap about 3.0 eV, and has a Vickers hardness 61.1 GPa lower than diamond but comparable with cubic boron nitride. Such a form of carbon, once obtained, would have wide applications in photocatalysis, adsoption, hydrogen storage and aerospace materials.

Keywords

Cite

@article{arxiv.1105.0977,
  title  = {T-Carbon: A Novel Carbon Allotrope},
  author = {Xian-Lei Sheng and Qing-Bo Yan and Fei Ye and Qing-Rong Zheng and Gang Su},
  journal= {arXiv preprint arXiv:1105.0977},
  year   = {2015}
}