Superconductivity in pressurized trilayer La$_4$Ni$_3$O$_{10-{\delta}}$ single crystals
Abstract
The pursuit of discovering new high-temperature superconductors that diverge from the copper-based paradigm1-3 carries profound implications for elucidating mechanisms behind superconductivity and may also enable new applications4-8. Here, our investigation reveals that application of pressure effectively suppresses the spin and charge order in trilayer nickelate La4Ni3O10-{\delta} single crystals, leading to the emergence of superconductivity with a maximum critical temperature (Tc) of around 30 K at 69.0 GPa. The DC susceptibility measurements confirm a substantial diamagnetic response below Tc, indicating the presence of bulk superconductivity with a volume fraction exceeding 80%. In the normal state, we observe a "strange metal" behavior, characterized by a linear temperature-dependent resistance extending up to 300 K. Furthermore, the layer-dependent superconductivity observed hints at a unique interlayer coupling mechanism specific to nickelates, setting them apart from cuprates in this regard. Our findings provide crucial insights into the fundamental mechanisms underpinning superconductivity, while also introducing a new material platform to explore the intricate interplay between the spin/charge order, flat band structures, interlayer coupling, strange metal behavior and high-temperature superconductivity.
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Cite
@article{arxiv.2311.07353,
title = {Superconductivity in pressurized trilayer La$_4$Ni$_3$O$_{10-{\delta}}$ single crystals},
author = {Yinghao Zhu and Di Peng and Enkang Zhang and Bingying Pan and Xu Chen and Lixing Chen and Huifen Ren and Feiyang Liu and Yiqing Hao and Nana Li and Zhenfang Xing and Fujun Lan and Jiyuan Han and Junjie Wang and Donghan Jia and Hongliang Wo and Yiqing Gu and Yimeng Gu and Li Ji and Wenbin Wang and Huiyang Gou and Yao Shen and Tianping Ying and Xiaolong Chen and Wenge Yang and Huibo Cao and Changlin Zheng and Qiaoshi Zeng and Jian-gang Guo and Jun Zhao},
journal= {arXiv preprint arXiv:2311.07353},
year = {2024}
}
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