We report Ru L3-edge resonant X-ray diffraction studies on single crystal and (001) epitaxial films of RuO2. We investigate the distinct Q=(100) and (001) reflections as a function of incident energy, azimuthal angle, and temperature. The results show that the observed resonant diffraction in RuO2 is fully consistent with a resonant charge anisotropy signal of structural origin permitted by the parent (non-magnetic) rutile P42/mnm space group. These results significantly constrain the magnetic contribution to the resonant diffraction signal and indicate the unlikely existence of k=0 antiferromagnetic order in RuO2.
@article{arxiv.2510.13767,
title = {Structural origin of resonant diffraction in RuO$_2$},
author = {Connor A Occhialini and Christie Nelson and Alessandro Bombardi and Shiyu Fan and Raul Acevedo-Esteves and Riccardo Comin and Dmitri N Basov and Maki Musashi and Masashi Kawasaki and Masaki Uchida and Hoydoo You and John Mitchell and Valentina Bisogni and Claudio Mazzoli and Jonathan Pelliciari},
journal= {arXiv preprint arXiv:2510.13767},
year = {2025}
}