We report magnetic susceptibility, isothermal magnetization, and specific-heat measurements on the rare-earth hexaaluminate SmMgAl11O19, where Sm3+ realizes a strongly quenched Kramers doublet on a triangular lattice with an exceptionally weak net exchange scale. The Curie--Weiss analysis yields strongly reduced ground-doublet g factors, gab≃0.65 and gc≃0.70. This indicates that the low-temperature response is governed primarily by single-ion physics, with crystal-field splitting and J-multiplet mixing jointly renormalizing the Sm3+ moment, rather than collective exchange. For H∥c, the specific heat shows no λ-type anomaly down to 0.35~K but evolves into a well-defined two-level Schottky peak whose gap grows linearly with field, yielding gc≃0.62 and recovering nearly all of Rln2 at high fields, thereby confirming an effective Seff=21 Kramers doublet description for T≲10~K. Together, these results establish SmMgAl11O19 as a weak-exchange, nearly single-ion triangular Kramers magnet in which frustration produce an anisotropic low-field correlated regime without inducing long-range order.
@article{arxiv.2601.13439,
title = {Strongly Quenched Kramers Doublet Magnetism in SmMgAl11O19},
author = {Sonu Kumar and Barbora Salajová and Andrej Kancko and Cinthia A. Corrêa and Shuvajit Halder and Ross H. Colman},
journal= {arXiv preprint arXiv:2601.13439},
year = {2026}
}