English

Strong laser alignment of solvent-solute aggregates in the gas-phase

Chemical Physics 2018-07-31 v2

Abstract

Strong quasi-adiabatic laser alignment of the indole-water-dimer clusters, an amino-acid chromophore bound to a single water molecule through a hydrogen bond, was experimentally realized. The alignment was visualized through ion and electron imaging following strong-field ionization. Molecular-frame photoelectron angular distributions showed a clear suppression of electron yield in the plane of the ionizing laser's polarization, which was analyzed as strong alignment of the molecular cluster with <cos2θ2D>\left< \cos^2\theta_{2D} \right> \ge 0.9.

Keywords

Cite

@article{arxiv.1801.08789,
  title  = {Strong laser alignment of solvent-solute aggregates in the gas-phase},
  author = {Sebastian Trippel and Joss Wiese and Terry Mullins and Jochen Küpper},
  journal= {arXiv preprint arXiv:1801.08789},
  year   = {2018}
}

Comments

7 pages, 3 figures