Strong intervalley correlation induced a magnetic order transition in monolayer $\text{MoS}_{2}$
Abstract
In this work, we study a model for monolayer molybdenum disulfide with including the intravalley and intervalley electron-electron interaction. We solve the model at a self-consistent mean-field level and get three solutions , and . As for , the spin polarizations are opposite at and valley and the total magnetization is zero. describe two degenerate spin-polarized states, and the directions of polarization are opposite for the states of and . Based on these results, the ground state can be deduced to be spin polarized in domains in which their particular states can be randomly described by or . Therefore, a zero net magnetization is induced for zero external magnetic field , but a global ferromagnetic ground state for a nonzero . We estimate the size of domains as several nanometers. As the increase of the chemical potential, the ground state changes between and , indicating first order phase transitions at the borders, which is coincident with the observation of photoluminescence experiments in the absence of the external magnetic field [J. G. Roch , Phys. Rev. Lett. , 187602 (2020)].
Keywords
Cite
@article{arxiv.2112.08664,
title = {Strong intervalley correlation induced a magnetic order transition in monolayer $\text{MoS}_{2}$},
author = {Peng Fan and Zhen-Gang Zhu},
journal= {arXiv preprint arXiv:2112.08664},
year = {2021}
}
Comments
12 pages, 6 figures