English

Strong coupling between a dielectric nanocavity and a monolayer transition metal dichalcogenide

Optics 2025-06-25 v2 Other Condensed Matter

Abstract

We demonstrate strong coupling between light in a dielectric nanocavity with deep sub-wavelength confinement and excitons in a monolayer of molybdenum ditelluride. Avoided crossing is demonstrated by both photoluminescence and reflection measurements, from which we extract a light-matter interaction strength of gPL=\SI5.3±0.3\milli\eVg_{\mathrm{PL}} =\SI{5.3\pm0.3}{\milli\eV} and gR=\SI4.7±0.7\milli\eVg_{\mathrm{R}} =\SI{4.7\pm0.7}{\milli\eV}, respectively. The associated Rabi splitting is twice as large as the system's losses. These values are in good agreement with values obtained by a novel exciton reaction coordinate formalism, yielding gtheory=\SI5.2±0.7\milli\eVg_{\mathrm{theory}} = \SI{5.2\pm0.7}{\milli\eV}. The strong light-matter interaction, combined with low losses and sub-wavelength confinement of light, black demonstrates a new regime of light-matter interactions where strong nonlinearities at the single-photon level are expected.

Keywords

Cite

@article{arxiv.2502.06529,
  title  = {Strong coupling between a dielectric nanocavity and a monolayer transition metal dichalcogenide},
  author = {F. Schröder and P. Wyborski and M. Xiong and G. Kountouris and B. Munkhbat and M. Wubs and P. T. Kristensen and J. Mørk and N. Stenger},
  journal= {arXiv preprint arXiv:2502.06529},
  year   = {2025}
}